1,119 results match your criteria: "and Institute of Physics[Affiliation]"

Recently, theoretical and experimental research predicted that ferromagnets with strong spin-orbit coupling (SOC) could serve as spin sources with dramatically enhanced spin-orbit torque (SOT) efficiency due to the combination of spin Hall effect and anomalous Hall effect (AHE), presenting potential advantages over conventional nonmagnetic heavy metals. However, materials with a strong SOC and room-temperature ferromagnetism are rare. Here, we report on a ferromagnetic (FM) interfacial phase with Curie temperature exceeding 300 K in the heavy transition-metal oxide CaRuO, in proximity to LaSrMnO.

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Pressure induced semiconductor-like to metal transition and linear magnetoresistance in CrSsingle crystal.

J Phys Condens Matter

November 2024

Beijing National Laboratory for Condensed Matter Physics, and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, People's Republic of China.

The transition metal chalcogenide CrShas unique properties, such as a lower antiferromagnetic transition temperature, semiconducting behavior, and thermoelectric properties. We focus on the effects of high pressure on the properties of electrical transport and structure in the single crystal CrS. It is observed that the resistance drops abruptly by approximately two orders of magnitude and the temperature derivative of the resistance changes from negative to positive after 15.

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The cascade of correlated topological quantum states in the newly discovered vanadium-based kagome superconductors, AVSb (A = K, Rb, and Cs), with a Z topological band structure has sparked immense interest. Here, we report the discovery of superconductivity and electronic nematic order in high-quality single-crystals of a new titanium-based kagome metal, CsTiBi, that preserves the translation symmetry, in stark contrast to the charge density wave superconductor AVSb. Transport and magnetic susceptibility measurements show superconductivity with an onset superconducting transition temperature T of approximately 4.

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Electronic and magnetic excitations in LaNiO.

Nat Commun

November 2024

National Synchrotron Radiation Laboratory and School of Nuclear Science and Technology, University of Science and Technology of China, Hefei, China.

High-temperature superconductivity was discovered in the pressurized nickelate LaNiO which has a unique bilayer structure and mixed valence state of nickel. The properties at ambient pressure contain crucial information of the fundamental interactions and bosons mediating superconducting pairing. Here, using X-ray absorption spectroscopy and resonant inelastic X-ray scattering, we identified that Ni 3 , Ni 3 , and ligand oxygen 2p orbitals dominate the low-energy physics with a small charge-transfer energy.

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Article Synopsis
  • * Researchers used advanced electron energy loss spectroscopy to identify new optical phonon modes that strongly interact with electrons, which are primarily due to vibrations of oxygen atoms in the interface layers.
  • * The results indicate a direct relationship between the strength of electron-phonon coupling and the distance between FeSe and the TiO-layer in SrTiO, offering insights into improving superconductivity in similar materials.
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High harmonic generation (HHG) have received significant attention for the exploration of material properties and ultrafast dynamics. However, the lack of consideration for couplings between HHG and other quasiparticles, such as phonons, has been impeding the understanding of many-body interactions in HHG. Here, we reveal the many-body electron-phonon mechanism in the quasiparticle-coupled strong-field dynamics by investigating the nonadiabatic (NA) coherent-phonon-coupled HHG.

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Engineering a Cu-Pd Paddle-Wheel Metal-Organic Framework for Selective CO Electroreduction.

Angew Chem Int Ed Engl

December 2024

Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry and TUM School of Natural Sciences, Technical University of Munich, Lichtenbergstraße 4, D-85748, Garching, Germany.

Article Synopsis
  • Optimizing the binding energy at active sites is essential for improving the selectivity and activity of catalysts in the electrochemical reduction of CO2. !* -
  • Copper is effective in reducing CO to hydrocarbons but struggles with product selectivity due to moderate binding energies of intermediates; a new Cu-Pd dimer structure is proposed using a metal-organic framework (MOF) to address this issue. !* -
  • The incorporation of palladium into the Cu-Pd structure enhances the adsorption of the COOH* intermediate, leading to more selective generation of carbon monoxide and deepening the understanding of catalyst structure-activity relationships. !*
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Lanthanide Functionalized Carbon Quantum Dots for White Light Emission, pH Sensing, and Co (II) Detection.

ACS Appl Mater Interfaces

November 2024

Engineering Research Center of Optical Instrument and System, Ministry of Education and Shanghai Key Laboratory of Modern Optical System, University of Shanghai for Science and Technology, Shanghai 200093, China.

Carbon quantum dots (CQDs) with fluorescence emission have been widely studied for versatile applications, but facile tunability of the spectral properties of CQDs by doping remains to be further explored. Herein, employing lanthanide ion Eu as a dopant and activator, a simple and efficient synthesis route for pure CQDs and Eu-CQDs was demonstrated using N, N-dimethylformamide, oleic acid, and oleylamine as precursors for carbon sources. In comparison, with the popular citric acid precursor, the as-prepared CQDs and Eu-CQDs exhibited an obviously smaller particle size (1.

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In structures with special geometry lattices, variations in stacking sequences are ubiquitous, yielding many novel structures and functionalities. Despite a wealth of intriguing properties and wide-ranging applications, there remains a considerable gap in understanding the correlation between special geometry lattices and functionalities in borides. Here, we design and synthesize a new superconducting boride NbIrB, with a body-centered orthorhombic structure, consisting of alternating two-dimensional [Nb-Ir-Nb] triple-triangular-lattice-layers and B fragment layers.

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Generalized Langevin subdiffusion in channels: The bath always wins.

Phys Rev E

September 2024

Institut für Physik and IRIS Adlershof, Humboldt-Universität zu Berlin, Newtonstraße 15, D-12489 Berlin, Germany.

We consider subdiffusive motion, modeled by the generalized Langevin equation in an equilibrium setting, of tracer particles in channels of indefinite length in the x direction: the channels of varying width and the channels with sinusoidally meandering midline. The subdiffusion in the x direction is not affected by constraints put by the channel. This is especially astonishing for meandering channels whose centerline might be quite long.

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The noble metal alloy AuSn has recently been identified as an intrinsic surface topological superconductor, promisingly hosting the Majorana zero mode (MZM) for topological quantum computing. However, the atomic visualization of its nontrivial surface states and MZM remains elusive. Here, we report the direct observation of unconventional surface states and vortex zero mode in AuSn by scanning tunneling microscopy/spectroscopy.

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Rhombohedral R3 Phase of Mn-Doped HfZrO Epitaxial Films with Robust Ferroelectricity.

Adv Mater

November 2024

State Key Lab of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084, China.

HfO-based ferroelectric materials are emerging as key components for next-generation nanoscale devices, owing to their exceptional nanoscale properties and compatibility with established silicon-based electronics infrastructure. Despite the considerable attention garnered by the ferroelectric orthorhombic phase, the polar rhombohedral phase has remained relatively unexplored due to the inherent challenges in its stabilization. In this study, the successful synthesis of a distinct ferroelectric rhombohedral phase is reported, i.

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Impact of Irreversible Adsorption on Molecular Ordering and Charge Transport in Poly(3-hexylthiophene) Thin Films on Solid Substrates.

ACS Appl Mater Interfaces

October 2024

Key Laboratory of Advanced Materials and Devices for Post-Moore Chips, Ministry of Education, School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, China.

Article Synopsis
  • - The study examines how the thermal annealing of poly(3-hexylthiophene) (P3HT) thin films on silicon dioxide substrates affects their crystalline structure and charge transport properties, noting that short-time annealing improves molecular ordering while long-time annealing disrupts it.
  • - Prolonged heat exposure leads to irreversible adsorption of P3HT chains at the polymer-solid interface, forming an amorphous layer that diminishes the film's overall crystallinity and disrupts ordering throughout the material.
  • - The research shows that optimal electrical performance in organic field-effect transistors (OFETs) is achieved with carefully timed annealing, balancing molecular ordering and the negative effects of chain adsorption, thereby enhancing charge carrier
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Article Synopsis
  • * The study investigates how laser-induced water plasma creates a favorable environment for hydrogen production using advanced simulations.
  • * Findings indicate that adjusting factors like annealing rate and laser wavelength can optimize hydrogen output, achieving an energy conversion efficiency of about 9.2%.
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Creating and unveiling chiral systems is important to the development of new materials and devices. In this study, after depositing prochiral radical molecule 3-carbamoyl-2,2,5,5-tetramethyl pyrroline-1-oxyl (CTPO) on a Au(111) substrate, 2D molecular crystals with two chiralities of CTPO molecules have been discovered. A single CTPO molecule is an achiral molecule in three-dimensional space, and it can form chiral configurations after adsorbing on the substrate.

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Article Synopsis
  • The Ruddlesden-Popper bilayer nickelate LaNiO has been linked to high-temperature superconductivity (HTSC) under high pressure (over 14 GPa), but lacks clear diamagnetic signals due to low superconducting volume fractions.
  • Research on Pr-doped LaPrNiO polycrystalline samples shows that Pr substitutions help create a nearly pure bilayer structure, mitigating the intergrowth of competing phases.
  • At pressures above 11 GPa, a transition occurs, with HTSC developing further, achieving notable superconducting transition temperatures and confirming bulk HTSC through significant diamagnetic signals below 75 K at over 15 GPa.
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Restoring Adiabatic State Transfer in Time-Modulated Non-Hermitian Systems.

Phys Rev Lett

September 2024

Theoretical Quantum Physics Laboratory, Cluster for Pioneering Research, RIKEN, Wako-shi, Saitama 351-0198, Japan.

Non-Hermitian systems have attracted much interest in recent decades, driven partly by the existence of exotic spectral singularities, known as exceptional points (EPs), where the dimensionality of the system evolution operator is reduced. Among various intriguing applications, the discovery of EPs has suggested the potential for implementing a symmetric mode switch, when encircling them in a system parameter space. However, subsequent theoretical and experimental works have revealed that dynamical encirclement of EPs invariably results in asymmetric mode conversion; namely, the mode switching depends only on the winding direction but not on the initial state.

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Excellent Barocaloric Effect by Modulating Geometrical Frustrations in MnPt.

J Am Chem Soc

October 2024

Department of Physical Chemistry, Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, China.

Article Synopsis
  • * Research highlights the large barocaloric effect (BCE) in MnPt, showing a significant temperature change strength of 9.77 K per 100 MPa, driven by low pressure and geometrical frustration.
  • * The study reveals that geometrical frustration enhances BCE by inducing strong spin fluctuations and magnetic moment changes, leading to greater sensitivity in magnetic phase transitions and advancing barocaloric refrigeration research.
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Spin texture in -space is a consequence of spin splitting due to strong spin-orbit coupling and inversion symmetry breaking. It underlies fertile spin transport phenomena and is of crucial importance for spintronics. Here, we observe the spin texture in -space of nominally centrosymmetric SrIrO grown on NdGaO (110) substrates, using non-linear magnetotransport measurements.

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Observation of Spin Splitting in Room-Temperature Metallic Antiferromagnet CrSb.

Adv Sci (Weinh)

November 2024

Department of Physics and Shenzhen Institute for Quantum Science and Engineering (SIQSE), Southern University of Science and Technology (SUSTech), Shenzhen, Guangdong, 518055, China.

Article Synopsis
  • Recent research has identified unconventional antiferromagnets that allow for spin splitting of electronic states, which could significantly advance antiferromagnetic spintronics due to their unique magnetic symmetries.
  • * The study focuses on CrSb, a promising metallic antiferromagnet with a high Néel temperature of 703 K, using techniques like angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) to analyze its electronic structure.
  • * Findings disclose a notable, k-dependent spin splitting of up to 0.8 eV, surpassing traditional spin-orbit coupling effects, suggesting CrSb could contribute to the development of efficient spintronic devices that work at room temperature.
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We present a new scheme for Majorana modes in systems with nonsymmorphic-symmetry-protected band degeneracy. We reveal that when the gapless fermionic excitations are encoded with conventional superconductivity and magnetism, which can be intrinsic or induced by proximity effect, topological superconductivity and Majorana modes can be obtained. We illustrate this outcome in a system which respects the space group P4/nmm and features a fourfold-degenerate fermionic mode at (π,  π) in the Brillouin zone.

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Artificial quantum systems have emerged as platforms to realize topological matter in a well-controlled manner. So far, experiments have mostly explored non-interacting topological states, and the realization of many-body topological phases in solid-state platforms with atomic resolution has remained challenging. Here we construct topological quantum Heisenberg spin lattices by assembling spin chains and two-dimensional spin arrays from spin-1/2 Ti atoms on an insulating MgO film in a scanning tunnelling microscope.

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Article Synopsis
  • The text discusses the theoretical and experimental challenges of achieving superconductivity in kagome materials, particularly highlighting nonmagnetic vanadium-based variants that do not support the expected exotic superconductivity.
  • A new chromium-based kagome metal, CsCrSb, is introduced, characterized by strong electron correlations, frustrated magnetism, and flat bands near the Fermi level.
  • This material undergoes a phase transition at 55 K, with density-wave orders evolving under pressure, leading to the emergence of superconductivity between 3.65-8.0 GPa, peaking at 6.4 K when these orders are suppressed, suggesting connections to unconventional superconductivity.
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CO capture and sequestration based on hydrate technology are considered supplementary approaches for reducing carbon emissions and mitigating the greenhouse effect. Direct CO hydrate formation and CH gas substitution in natural gas hydrates are two of the main methods used for the sequestration of CO in hydrates. In this Review, we introduce the crystal structures of CO hydrates and CO-mixed gas hydrates and summarize the interactions between the CO molecules and clathrate hydrate/HO frames.

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Superconductivity involving finite-momentum pairing can lead to spatial-gap and pair-density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here we detect chiral kagome superconductivity modulations with residual Fermi arcs in KVSb and CsVSb using normal and Josephson scanning tunnelling microscopy down to 30 millikelvin with a resolved electronic energy difference at the microelectronvolt level.

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