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Accurate strain monitoring in environments with coexisting mechanical deformation and temperature fluctuations─such as solid rocket propellants, battery enclosures, and human ligaments─remains a longstanding challenge for flexible electronics. Conventional strain sensors suffer from significant thermal drift due to the intrinsic temperature dependence of their sensing materials, limiting their reliability in wireless and implantable applications. Here, we report an intrinsically temperature-insensitive, highly sensitive, wireless flexible strain sensor based on near-field communication technology. We innovatively design and demonstrate a flexible strain sensor that simultaneously achieves low temperature drift, high sensitivity, and passive wireless functionality. By combining two engineered materials with opposing temperature coefficients of resistance, the device achieves self-compensated thermal stability with a minimal temperature drift of 160 × 10 °C, eliminating the need for external calibration. It exhibits an exceptionally high gauge factor of 2415.76 across a wide strain range (0-80%), and enables wireless, battery-free strain readout over a distance of 3 cm. We demonstrate the sensor's robust performance across three thermo-mechanically coupled scenarios: (1) strain monitoring within solid rocket motor propellant grains, (2) detection of volumetric deformation in lithium-ion batteries, and (3) ligament strain sensing in the human knee joint. This work provides a generalizable strategy for achieving thermal invariance in high-performance flexible strain sensors and expands the utility of passive wireless sensing in harsh and dynamic environments.
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http://dx.doi.org/10.1021/acssensors.5c01861 | DOI Listing |
Langmuir
September 2025
Department of Light Chemical Engineering, School of Textiles Science and Engineering; Key Laboratory of Special Protective, Ministry of Education; Jiangnan University, Wuxi 214122, P. R. China.
Polymerizable deep eutectic solvents (PDES) have recently emerged as a class of solvent-free ionically conductive elastomers and are considered among the most feasible candidates for next-generation ionotronic devices. However, the fundamental challenge persists in synergistically combining high mechanical strength, robust adhesion, reliable self-healing capacity, and effective antimicrobial performance within a unified material system capable of fulfilling the rigorous operational demands of next-generation ionotronic devices across multifunctional applications. Inspired by the hierarchical structure of spider silk, HCAG eutectogels composed of acrylic acid (AA), 2-hydroxyethyl acrylate (HEA), and choline chloride (ChCl) were successfully synthesized via a one-step photopolymerization method.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
Department of Mechanical Engineering, State University of New York at Binghamton, Binghamton, New York 13902, United States.
Soft conductive composites are significant components of soft and wearable electronics. Existing soft conductive composites encounter difficulties in attaining 10% of copper's electrical conductivity while maintaining high stretchability. In this work, a novel "soft conductive junction" concept is introduced to overcome the conductivity-stretchability trade-off.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
School of Physics, Nanjing University of Science and Technology, Nanjing 210094, China.
Multifunctional materials that simultaneously possess intrinsic magnetic and superhard properties, particularly those composed of light elements, have a wide range of applications in advanced sensors, shielding, durable devices, and other fields. However, research on the development and understanding of such materials remains limited. In this study, a series of 3D C covalent networks derived from the C fullerene precursor were theoretically designed.
View Article and Find Full Text PDFNano Lett
September 2025
School of Materials and Chemistry, University of Shanghai for Science & Technology, Shanghai 200093, China.
Developing low-temperature gas sensors for parts per billion-level acetone detection in breath analysis remains challenging for non-invasive diabetes monitoring. We implement dual-defect engineering via one-pot synthesis of Al-doped WO nanorod arrays, establishing a W-O-Al catalytic mechanism. Al doping induces lattice strain to boost oxygen vacancy density by 31.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
DUT School of Software Technology & DUT-RU International School of Information Science and Engineering, Dalian University of Technology, Dalian 116620, China.
Achieving both high sensitivity and a wide detection range in flexible pressure sensors poses a challenge due to their inherent trade-off. Although porous structures offer promising solutions, conventional methods (templating, foaming, and freeze-drying) fail to precisely control cavity dimensions, spatial arrangement, and 3D morphology, which are crucial for sensing performance. Here, we propose a scalable fabrication strategy that integrates triply periodic minimal surface (TPMS) geometries─precisely engineered via FDM 3D printing─with ultrasonic impregnation of carbon black (CB) into TPU scaffolds.
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