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The design of electrically conductive textiles appears to be a promising approach to combat the existing challenge of deaths caused by severe cold climates around the globe. However, reports on the scalable fabrication of tolerant conductive textiles maintaining a low electrical resistance with an ability for unperturbed and prolonged performance are scarce. Here, a breathable and wrappable water-repellent conductive textile (water-repellent CT) with electrothermal and photothermal conversion abilities at low external voltage and in weak solar light is introduced, respectively. In the current approach, less carbon-containing silver nanowires (AgNWs) are selected to spray deposit on a commercially available woven textile to attend a uniform and highly conductive network over a large dimension. The subsequent spray deposition of a reaction mixture of selected small molecules prevents aerial oxidation of deposited AgNWs even at elevated temperatures and provides bioinspired extreme water-repellence. Thus, it maintains an unperturbed performance even when exposed to different aqueous environment. Using the scalability of current approach and durability of prepared water-repellent CT, relevant wearable devices are derived to demonstrate personal heat management ability with rechargeable and portable battery for prolonged duration in severely cold conditions. Thus, the prepared water-repellent CT enabled an energy-efficient and "wrappable" heating, providing a basis for various potential applications.
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http://dx.doi.org/10.1002/smll.202412741 | DOI Listing |
Langmuir
September 2025
College of Textile and Clothing Engineering, Soochow University, Suzhou 215123, PR China.
Sodium-ion batteries are promising candidates for large-scale energy storage due to their low cost and resource abundance. However, their cathode materials suffer from poor conductivity and limited cycling stability. Here, we report a Prussian blue (PB)-based cathode hybridized with carboxyl-functionalized carbon nanotubes (CNTs) via a glutamic acid-assisted in situ coordination route.
View Article and Find Full Text PDFAdv Mater
September 2025
Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou, 215123, P. R. China.
Despite significant advancements in aerogels science, the fabrication of high-performance aerogels with their plastic processability remains unexplored owing to their inherent trade-off between skeletal rigidity and transformable processability. Herein, a universal solubility-pKa coupling-effect to engineer high-performance thermoplastic nylon aerogel family with excellent thermomechanical processing performance is proposed. By modulating solubility parameters and acid dissociation constants in nylon-solvent systems, it is precisely control crystallization to assemble interlaced 1D nanofiber skeletons, yielding nylon aerogels that integrate a high specific surface area (226 m g), exceptional compressive modulus (12.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
DUT School of Software Technology & DUT-RU International School of Information Science and Engineering, Dalian University of Technology, Dalian 116620, China.
Achieving both high sensitivity and a wide detection range in flexible pressure sensors poses a challenge due to their inherent trade-off. Although porous structures offer promising solutions, conventional methods (templating, foaming, and freeze-drying) fail to precisely control cavity dimensions, spatial arrangement, and 3D morphology, which are crucial for sensing performance. Here, we propose a scalable fabrication strategy that integrates triply periodic minimal surface (TPMS) geometries─precisely engineered via FDM 3D printing─with ultrasonic impregnation of carbon black (CB) into TPU scaffolds.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu 610065, China.
Gel-based electronic skin (e-skin) has recently emerged as one of the most promising interfaces for human-machine interaction and wearable devices, owing to its exceptional flexibility, extensibility, transparency, biocompatibility, high-quality physiological signal monitoring, and system integration suitability. However, conventional hydrogel-based e-skins may exhibit limitations in mechanical strength and stretchability compatibility, as well as poor environmental stability. To address these challenges, following a top-down fabrication strategy, this study innovatively integrates poly(methacrylic acid), titanium sulfate, and ethylene glycol (EG) into the three-dimensional collagen fiber network structure of zeolite-tanned sheepskin to successfully develop an organogel (SMEMT) e-skin, which exhibits superior high toughness, environmental stability, high transparency (74% light transmittance at 550 nm), antibacterial properties and ecological compatibility.
View Article and Find Full Text PDFMacromol Rapid Commun
September 2025
School of Materials and Chemistry, Anhui Agricultural University, Hefei, Anhui, China.
At present, flexible sensors are a hot spot in research and experimental development, but the research on flexible sensors that can be used for human motion monitoring still needs to be deepened. In this work, the green material cellulose acetate (CA) was used as the matrix material, the film was made by electrospinning, crushed by a cell grinder and sodium alginate (SA) was added to promote the uniform dispersion of nanofibers in water, and then methyltrimethoxysilane (MTMS) and MXene nanosheet dispersion were added to make it hydrophobic and good conductivity, and the aerogel precursor solution was prepared, and then the CA/SA/MTMS/MXene aerogel with directional holes was prepared by directional freeze-drying. As a flexible sensor material, it can be used for human wear, monitoring the electrical signals generated by the movement of human joints and other parts, and can still maintain a current of about 0.
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