Electronic structure modulation single atom interfacial engineering for selective atmospheric CO photoreduction.

Chem Commun (Camb)

State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control, School of Environmental Science and Engineering, Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control, Southern University of Science and Technology, Shenzhen, Guangdong

Published: November 2024


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Article Abstract

Single-atom iridium was interfacially engineered on CuFeS quantum dots (QDs) with highly efficient CO photoreduction performance. The electronic structure modulation yielded a remarkable CO yield rate of 32.5 μmol g h with 92.2% selectivity under atmospheric conditions. This work demonstrates the potential of single-atom interfacial engineering for advancing CO photoreduction.

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http://dx.doi.org/10.1039/d4cc05372aDOI Listing

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