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2D van der Waals (vdW) ferromagnets have emerged as promising materials for spintronic applications due to their unique magnetic properties and tunability. Controlling ferromagnetism via external stimuli is critical for both fundamental research and device integration. In particular, modulation of magnetic anisotropy and exchange interactions through strain offers a viable pathway for functional control. Owing to their weak interlayer coupling, vdW ferromagnets exhibit pronounced sensitivity to strain, enabling effective tuning of their magnetic states. In this study, electric-field-induced magnetoelectric coupling is investigated in the above-room-temperature vdW ferromagnet FeGaTe integrated on a ferroelectric PMN-PT substrate. It is demonstrated that application of an electric field leads to a substantial reduction in coercive force along with dynamic reconfiguration of the magnetic domain structure. These effects are attributed to electric-field-induced modulation of the vdW interlayer gap and enhancement of the Dzyaloshinskii-Moriya interaction. These findings reveal a strong interplay between electric fields and magnetism in vdW systems, offering a viable route toward the development of low-power, multifunctional magnetic devices. This work establishes a foundation for the electric-field control of magnetic properties in vdW ferromagnets and highlights their potential in next-generation spintronic technologies.
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http://dx.doi.org/10.1002/advs.202503530 | DOI Listing |
J Phys Condens Matter
September 2025
Wuhan University, Wuhan University, Wuhan, 430072, CHINA.
Manipulating magnetism in two-dimensional (2D) van der Waals (vdW) materials arouses considerable and ongoing interest in fundamental physics and potential applications in next-generation spintronics. Here, we have investigated the underlying electronic structures of bulk vdW magnets CrTe2 and NaCrTe2, by carrying out high-resolution angle-resolved photoemission spectroscopy (ARPES) studies and first-principles calculations. In CrTe2, strong out-of-plane band dispersions and metallic Fermi surface are observed, accompanied by temperature-dependent ferromagnetic (FM) energy gain behavior which directly confirms its itinerant origin.
View Article and Find Full Text PDFJ Am Chem Soc
September 2025
Department of Chemistry, Princeton University, Princeton, New Jersey 08544, United States.
Layered van der Waals (vdW) materials, characterized by their interlayer vdW gaps, offer exceptional tunability of magnetic properties via intercalation chemistry. A wide range of magnetic behaviors have been observed in nonmagnetic transition-metal dichalcogenides intercalated with magnetic atoms. Beyond the incorporation of magnetic ions, we propose the controlled alkali-ion intercalation of intrinsic vdW magnets as a strategy to probe and manipulate spin populations and exchange interactions within individual magnetic layers.
View Article and Find Full Text PDFACS Nano
September 2025
Ultrafast Electron Microscopy Laboratory, The MOE Key Laboratory of Weak-Light Nonlinear Photonics, School of Physics, Nankai University, Tianjin 300071, China.
Superlattices (SLs) based on two-dimensional (2D) van der Waals (vdW) materials, abbreviated as 2D-SLs, have garnered significant attention due to their customizable properties. 2D-SLs can be engineered by mechanical stacking or chemical intercalation to achieve diverse forms of symmetry breaking, resulting in exotic phenomena like the quantum anomalous Hall effect and topological magnetism. Hitherto, broken symmetries in 2D-SLs have been widely produced within lateral planes or three dimensions.
View Article and Find Full Text PDFAdv Sci (Weinh)
August 2025
Department of Physics, Kyushu University, 744 Motooka, Fukuoka, 819-0395, Japan.
2D van der Waals (vdW) ferromagnets have emerged as promising materials for spintronic applications due to their unique magnetic properties and tunability. Controlling ferromagnetism via external stimuli is critical for both fundamental research and device integration. In particular, modulation of magnetic anisotropy and exchange interactions through strain offers a viable pathway for functional control.
View Article and Find Full Text PDFNanomaterials (Basel)
August 2025
College of Physics Science and Technology, Yangzhou University, Yangzhou 225002, China.
Photocatalytic water splitting for hydrogen production is an attractive renewable energy technology, but the oxygen evolution reaction (OER) at the anode is severely constrained by a high overpotential. The two-dimensional vdW ferromagnetic material FeGeTe, with its good stability and excellent metallic conductivity, has potential as an electrocatalyst, but its sluggish surface catalytic reactivity limits its large-scale application. In this work, we adapted DFT calculations to introduce surface Te vacancies to boost OER performance of the FeGeTe (001) surface.
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