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The development of wearable strain sensors for the human-machine interface has attracted considerable research interest. Most existing wearable strain sensors were incapable of simultaneously detecting strain amplitudes and directions, and they failed to fully record stretching vectors that occurred on the body. Graphene and graphene-derived materials have been utilized to construct wearable strain sensors with excellent electrical sensitivities. Although the growth techniques of planar graphene and vertical graphene (VG) have been established, the fabrication of VG aligned in parallel within a larger area has not been previously achieved. Here, parallelly aligned VG (PAVG) in a large area was successfully fabricated and constructed as a wearable strain vector sensor. The PAVG was fabricated via inductively coupled plasma chemical vapor deposition assisted by metal inducers. The as-fabricated sensor was electrically anisotropic because of the profiles of the VG nanosheets aligned in parallel. Therefore, the sensor could simultaneously and sensitively detect the direction and the amplitude of the strain vectors with excellent accuracy. Application of this strain vector sensor for the human-sensor interface to identify the stretching directions and amplitudes of finger joints was also demonstrated. This work established the fabrication methodology of graphene with unique vertical and parallel alignment morphology. This study introduced a new opportunity of developing wearable sensors that could fully detect multidirectional human actions.
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http://dx.doi.org/10.1021/acsami.8b18210 | DOI Listing |
J Colloid Interface Sci
September 2025
Research Center of Nano Science and Technology, College of Sciences, Shanghai University, Shanghai 200444, PR China. Electronic address:
Ionic conductive hydrogels show promise for flexible sensors in wearables and e-skins, but balancing mechanical strength with high conductivity remains challenging. Herein, a triple-network ionic conductive hydrogel based on poly(acrylic acid) (PAA) was developed, synergistically reinforced by dissolved cellulose (dCel) and aramid nanofibers (ANF), with Al/Zn bimetallic ions serving as the conductive medium. Intriguingly, dCel was in-situ generated using the concentrated Al/Zn bimetallic salt solutions as the cellulose solvent, following the complete dissolution of the pulp fibers driven by the intensive ionic hydration of Al/Zn ions.
View Article and Find Full Text PDFLangmuir
September 2025
Department of Light Chemical Engineering, School of Textiles Science and Engineering; Key Laboratory of Special Protective, Ministry of Education; Jiangnan University, Wuxi 214122, P. R. China.
Polymerizable deep eutectic solvents (PDES) have recently emerged as a class of solvent-free ionically conductive elastomers and are considered among the most feasible candidates for next-generation ionotronic devices. However, the fundamental challenge persists in synergistically combining high mechanical strength, robust adhesion, reliable self-healing capacity, and effective antimicrobial performance within a unified material system capable of fulfilling the rigorous operational demands of next-generation ionotronic devices across multifunctional applications. Inspired by the hierarchical structure of spider silk, HCAG eutectogels composed of acrylic acid (AA), 2-hydroxyethyl acrylate (HEA), and choline chloride (ChCl) were successfully synthesized via a one-step photopolymerization method.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
Department of Mechanical Engineering, State University of New York at Binghamton, Binghamton, New York 13902, United States.
Soft conductive composites are significant components of soft and wearable electronics. Existing soft conductive composites encounter difficulties in attaining 10% of copper's electrical conductivity while maintaining high stretchability. In this work, a novel "soft conductive junction" concept is introduced to overcome the conductivity-stretchability trade-off.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
September 2025
McKetta Department of Chemical Engineering, The University of Texas at Austin, Austin, TX 78712.
Many soft, tough materials have emerged in recent years, paving the way for advances in wearable electronics, soft robotics, and flexible displays. However, understanding the interfacial fracture behavior of these materials remains a significant challenge, owing to the difficulty of quantifying the respective contributions from viscoelasticity and damage to energy dissipation ahead of cracks. This work aims to address this challenge by labeling a series of polymer networks with fluorogenic mechanophores, subjecting them to T-peel tests at various rates and temperatures, and quantifying their force-induced damage using a confocal microscope.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
DUT School of Software Technology & DUT-RU International School of Information Science and Engineering, Dalian University of Technology, Dalian 116620, China.
Achieving both high sensitivity and a wide detection range in flexible pressure sensors poses a challenge due to their inherent trade-off. Although porous structures offer promising solutions, conventional methods (templating, foaming, and freeze-drying) fail to precisely control cavity dimensions, spatial arrangement, and 3D morphology, which are crucial for sensing performance. Here, we propose a scalable fabrication strategy that integrates triply periodic minimal surface (TPMS) geometries─precisely engineered via FDM 3D printing─with ultrasonic impregnation of carbon black (CB) into TPU scaffolds.
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