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Soft capacitive strain sensors with soft conductive electrodes are advantageous for their ability to decouple resistance from the flexible electrodes, offering excellent repeatability, low hysteresis, low energy consumption, and good temperature stability. However, existing soft capacitive strain sensors utilize intrinsically stiff conductors as soft electrodes, limiting the sensitivity, repeatability, and hysteresis. To address these issues, this work proposes a soft capacitive strain sensor based on liquid metal. The soft electrodes are composed of a liquid metal-nickel particle conductive paste, which combines fluidity and low surface tension, thereby eliminating the elastic modulus mismatch between the soft electrodes and the elastomers. This design achieves high sensitivity, excellent repeatability, and low hysteresis. The sensor employs a three-electrode structure, which enhances resistance to parasitic and stray capacitance without applying shielding layers. The measurement and the self-shielding of the three-electrode structure are investigated through simulation analyses. Additionally, the influence of the elastic modulus compatibility between the soft electrodes and the elastomers is investigated through experiments and simulations. Furthermore, the application of this sensor in the field of wearable devices is demonstrated.
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http://dx.doi.org/10.1021/acsami.5c10267 | DOI Listing |
CuZnSnS (CZTS) has been synthesised using ethylene glycol as a solvent by the solvothermal method. Preliminary characterisation, like X-ray diffraction, Raman spectroscopy, and FTIR, confirmed the tetragonal structure of CZTS with kesterite phase. In the synthesis, a series of samples with different concentrations of sulfur were produced, accompanied by an in-depth analysis of structural parameters such as crystallite size and strain, utilising both the Scherrer equation and the Williamson-Hall method.
View Article and Find Full Text PDFACS Nano
September 2025
College of Materials Science and Engineering, Hunan University, Changsha 410082, China.
The development of high-mass-loading electrodes offers a promising solution for enhancing energy density and reducing costs by minimizing inactive components. However, thick electrodes often face challenges, such as structural instability and poor electron and ion transport. Here, we present a strain-induced strategy for preparing distorted MXene nanosheets, enabling the fabrication of pressure-resistant crumpled freestanding electrodes with low tortuosity and a curvature-induced cation enrichment effect.
View Article and Find Full Text PDFACS Appl Mater Interfaces
August 2025
Institute of Fundamental Technological Research, Polish Academy of Sciences, Pawinskiego 5B Str., 02-106 Warsaw, Poland.
For the development of next-generation portable energy storage devices, compression-tolerant electrodes are essential, but most of the previous reports have focused only on carbon-based materials. Herein, gelatin methacrylate (GelMA) and poly(-isopropylacrylamide) (PNIIPAM) were used as hosts to incorporate the CoO@MoS aerogel (CoO@MoS AG). GelMa-PNIPAM (GP) was transformed into a carbon network as an intrinsically compressible host template with high conductivity.
View Article and Find Full Text PDFAdv Sci (Weinh)
August 2025
College of Mechanical Engineering, Yangzhou University, Yangzhou, 225127, China.
The additive manufacturing of micro-supercapacitors (MSCs) with outstanding areal energy density and scalable integration remains challenging due to the incompatibility between printability and functionality of electronic ink. Here, a thixotropic MXene/conductive cellulose heteroink is formulated, eliminating the need for tedious processing and toxic organic additives, to construct MSCs with high areal energy density. Conductive cellulose with radially graded structure containing defect-rich graphitic shells not only inhibits MXene re-stacking through hydrogen-bonded 3D porous networks, but also establishes sp-carbon pathways for rapid electron transport.
View Article and Find Full Text PDFAdv Mater
August 2025
Faculty of Materials Science and Chemistry, China University of Geosciences, 388 Lumo Road, Wuhan, 430074, P. R. China.
Owing to the unique mechano-optical response, mechanoluminescence (ML) materials possess dynamic, sensitive, visual, and recoverable strain sensing capabilities. However, the dilemma of lacking outstanding ML materials with high detection precision under micro deformations still exists, thereby hindering advanced applications in multi-angle and multidimensional scenarios. Herein, a novel Pr-doped perovskite oxide (NaTaO:Pr)-based composite elastic thin film is developed, which achieves ultrasensitive ML responses to both microscale compressive and tensile strains.
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