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Lack of access to sanitation is a challenge that persists globally, with low sewerage connection rates in many low- and lower-middle-income countries. Engineered nonsewered sanitation (NSS) technologies can meet treatment requirements without sewers, but their relative sustainability varies across potential deployment sites. Here, we characterize the costs and carbon intensity (CI) of three emerging NSS technologies, two community reinvented toilets (CRTs) and one Omni Processor (OP), across 77 countries, identify sustainability performance typologies, and map typology prevalence in countries across the globe. Locality-specific factors such as wages, diet, and material costs drive regional variability in NSS costs by up to 15-fold and CI up to 2-fold within technologies. Across all three NSS technologies and all scenarios evaluated, costs ranged from 0.01 to 0.36 USD·capita·day and CIs ranged from 8 to 269 kg CO eq·capita·year. Low-cost, low-CI typologies are predominantly in countries with lower human development indices (HDI 2-4), demonstrating alignment between the sanitation need and the NSS opportunity space. Ultimately, the intent of this work is not to imply one-size-fits-all solutions for individual countries; by elucidating key sustainability drivers and defining typologies, this work can support early-stage decision-making for NSS technology research, development, and deployment.
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http://dx.doi.org/10.1021/acs.est.5c02064 | DOI Listing |
Small
September 2025
Centre for Interdisciplinary Research, D. Y. Patil Education Society (Deemed to be University), Kolhapur, Maharashtra, 416 006, India.
Developing efficient, sustainable, earth-abundant, cost-effective electrocatalysts is extremely challenging. Cobalt-iron-layered double hydroxide nanosheets (Co-Fe-LDH NSs) hybridized with carbon nanotubes (CNTs) lead to anchors Co-Fe-LDH-CNTs (CFC) self-assembly with a mesoporous morphology, expanded surface area, fast charge transfer kinetics, and high electrical conductivity. The resultant anchored CFC nanohybrid is highly active for electrocatalytic oxygen evolution reaction (OER), showing a lower overpotential of 221 and 313 mV at a current density of 10 and 25 mA cm, respectively, compared to pristine Co-Fe-LDH (339 and 391 mV), showcasing the significant role of CNTs in improving the electrocatalytic performance of pristine Co-Fe-LDH.
View Article and Find Full Text PDFAnal Chem
September 2025
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, Jiangsu 213164, P. R. China.
Rational design of both mechanistic pathways and material compositions is essential to advance COF-based electrochemiluminescence (ECL) systems. In this study, aggregation-induced emission covalent organic framework (AIE-COF) nanoprobes with excellent ECL performance were developed based on Tb-functionalized covalent organic framework (Tb@A-COF). The Tb@A-COF system demonstrates enhanced ECL performance through synergistic integration of three complementary mechanisms: (1) (4',4',4',4'-(1,2-ethenediylidene)tetrakis [1,1'-biphenyl]-4-carboxaldehyde (ETBC) ligands function as antenna-like sensitizers that amplify luminescence intensity by 14.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
September 2025
State Key Laboratory of Food Science and Technology, School of Food Science and Technology, Jiangnan University, Wuxi, Jiangsu, 214122, China.
All inorganic lead halide perovskite (CsPbX) has become a hot topic in chiral optics for its high quantum yield and tunable luminescence. The environmental degradation tendency and lack of magneto-optical coupling mechanism of lead-based perovskite severely restrict its chirality integrated application. Rare-earth ions (such as Gd, Eu), with their unique 4f electronic configuration, not only passivate the lattice defects to improve stability but also expand the spectral response range through electronic localization effects.
View Article and Find Full Text PDFAdv Mater
August 2025
Key Laboratory of Superlight Materials and Surface Technology, Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin, 150001, P. R. China.
Thermoelectric technology, a rapidly advancing field in medical therapy, encounters challenges in achieving efficient thermal and electrical transport properties within the limited thermal range compatible with biological systems. This study presents a high-performance thermoelectric catalytic therapy (TECT) utilizing Cu self-doped CuZnSnSe nanosheets synthesized with non-stoichiometric ratios modified with DSPE-mPEG (n-CZTSe@PEG NSs). Under 808 nm laser irradiation, n-CZTSe@PEG NSs demonstrate an impressive photothermal conversion efficiency of 47.
View Article and Find Full Text PDFNanomicro Lett
August 2025
Department of Chemistry and Nanoscience, Ewha Womans University, 52 Ewhayeodae-Gil, Seodaemun-Gu, Seoul, 03760, Republic of Korea.
Lithium-oxygen (Li-O) batteries are perceived as a promising breakthrough in sustainable electrochemical energy storage, utilizing ambient air as an energy source, eliminating the need for costly cathode materials, and offering the highest theoretical energy density (~ 3.5 kWh kg) among discussed candidates. Contributing to the poor cycle life of currently reported Li-O cells is singlet oxygen (O) formation, inducing parasitic reactions, degrading key components, and severely deteriorating cell performance.
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