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Plastics are ubiquitous in today's lifestyle, and their indiscriminate use has led to the accumulation of plastic waste in landfills and oceans. The waste accumulates and breaks into micro-particles that enter the food chain, causing severe threats to human health, wildlife, and the ecosystem. Environment-friendly and bio-based degradable materials offer a sustainable alternative to the vastly used synthetic materials. Here, a polylactic acid and carbon nanofiber-based membrane and a paper-based colorimetric sensor have been developed. The membrane had a surface area of 3.02 m g and a pore size of 18.77 nm. The pores were evenly distributed with a pore volume of 0.0137 cm g. The membrane was evaluated in accordance with OECD guidelines and was found to be safe for tested aquatic and terrestrial models. The activated PLA-CNF membrane was further used as a bio-based electrode for the electrochemical detection of nitrates (NO) in water samples with a detection limit of 0.046 ppm and sensitivity of 1.69 × 10 A ppm mm, whereas the developed paper-based colorimetric sensor had a detection limit of 156 ppm for NO. This study presents an environment-friendly, low-carbon footprint disposable material for sensing applications as a sustainable alternative to plastics.
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http://dx.doi.org/10.1039/d3ay02069j | DOI Listing |
Anal Chim Acta
November 2025
Department of Physics, University of Lucknow, Lucknow, India; Department of Physics and Astrophysics, University of Delhi, India. Electronic address:
Background: Water contamination is a global challenge, primarily due to heavy metal ions like lead (Pb), iron (Fe), cadmium (Cd), andmercury (Hg) as well as dyes. These pollutants enter the ecosystem from industrial waste and runoff, accumulate in the environment and pose a high risk to humans, animals and plants. Various sensors, such as colorimetric sensors, and electrochemical sensors have been developed to detect these ions and dyes.
View Article and Find Full Text PDFAnal Chim Acta
November 2025
NHC Key Laboratory of Tropical Disease Control, School of Tropical Medicine, Hainan Medical University, Haikou, Hainan, 571199, China. Electronic address:
Background: While paper-based colorimetric assays have seen significant progress in recent years, persistent challenges including the coffee-ring effect and infiltration effect continue to affect the color uniformity of detection results, leading to decreased sensitivity and accuracy of the detection. Recent advancements in suppressing these two effects mainly depend on chemical modification of cellulose fibers or application of specific functional coatings. However, the former's complex procedures impede large-scale implementation, while the latter's non-cellulosic additives risk unpredictable interactions with analytes or interference in colorimetric reactions.
View Article and Find Full Text PDFMetal nanoparticles (MNPs) have emerged as vital components in nanotechnology due to their unique ability to concentrate light at the nanoscale. This property makes them especially valuable in biosensing applications, where high sensitivity is essential. At the same time, cellulose-based materials like paper offer an affordable, widely available, and versatile platform, making them ideal for the development of paper-based microfluidic analytical devices (μPADs).
View Article and Find Full Text PDFAnal Chem
September 2025
State Key Laboratory of Green Chemical Synthesis and Conversion, College of Chemical Engineering, Zhejiang University of Technology, Hangzhou 310032, PR China.
Residues of organophosphorus pesticides (OPs) raise considerable concern, while achieving high enough detection sensitivity is still a challenge for on-site fluorescence techniques. Herein, we report a "double-end samplification" strategy by encapsulating a low-emission fluorescent ion probe [DCF][P] into a cetyltrimethylammonium bromide (CTAB) hydrophobic core to form ionic luminescent micelles. At the probe end, ionic liquid micelles locally concentrated the probes, achieving a 350-fold fluorescence enhancement.
View Article and Find Full Text PDFAdv Healthc Mater
September 2025
Hubei Engineering Technology Research Center of Spectrum and Imaging Instrument, Electronic Information School, Wuhan University, Wuhan, 430072, China.
Accurate and rapid detection of urinary creatinine (CR) is critical for early kidney disease screening and efficient healthcare resource management. In this study, a novel colorimetric-fluorescent sensor is developed by integrating nitrogen-doped carbon dots (N-CDs) and copper nanoclusters (CuNCs) with gold nanoparticles (AuNPs), leveraging fluorescence resonance energy transfer (FRET) to enhance sensitivity and selectivity. The sensor functions within a detection range of 1-50 mm, with peak responsiveness at 17 mm, utilizing paper-based substrates for a low-cost and portable application.
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