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Antiferromagnets constitute promising contender materials for next-generation spintronic devices with superior stability, scalability, and dynamics. Nevertheless, the perception of well-established ferromagnetic spintronics underpinned by spontaneous magnetization seemed to indicate the inadequacy of antiferromagnets for spintronics-their compensated magnetization has been perceived to result in uncontrollable antiferromagnetic order and subtle magnetoelectronic responses. However, remarkable advancements have been achieved in antiferromagnetic spintronics in recent years, with consecutive unanticipated discoveries substantiating the feasibility of antiferromagnet-centered spintronic devices. It is emphasized that, distinct from ferromagnets, the richness in complex antiferromagnetic crystal structures is the unique and essential virtue of antiferromagnets that can open up their endless possibilities of novel phenomena and functionality for spintronics. In this Perspective, the recent progress in antiferromagnetic spintronics is reviewed, with a particular focus on that based on several kinds of antiferromagnets with special antiferromagnetic crystal structures. The latest developments in efficiently manipulating antiferromagnetic order, exploring novel antiferromagnetic physical responses, and demonstrating prototype antiferromagnetic spintronic devices are discussed. An outlook on future research directions is also provided. It is hoped that this Perspective can serve as guidance for readers who are interested in this field and encourage unprecedented studies on antiferromagnetic spintronic materials, phenomena, and devices.
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http://dx.doi.org/10.1002/adma.202310379 | DOI Listing |
Adv Mater
September 2025
State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai, 200433, China.
Superconductivity and magnetism are two of the most extensively studied ordered systems in condensed matter physics. Recent advancements in the fabrication of van der Waals (vdW) layered materials have significantly advanced the exploration of both fundamental physics and practical applications within their heterostructures. The focus not only lies on the coexisting mechanism between superconductivity and magnetism, but also highlights the potential of these atomically thin layers to serve as crucial components in future superconducting circuits.
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August 2025
School of Physics, Nanjing University of Science and Technology Nanjing 210094 China
The role of electronic spin in electrocatalysis has led to the emerging field of "spin-dependent electrocatalysis". While spin effects in individual active sites have been well understood, spin coupling among multiple sites remains underexplored in electrocatalysis, which will bring forth new active sites and mechanisms. In this work, we propose a general theory to understand the spin coupling in electrocatalysis.
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September 2025
Department of Semiconductor Physics and Institute of Quantum Convergence Technology, Kangwon National University, Chuncheon, 24341, South Korea.
2D van der Waals ferromagnets hold immense promise for spintronic applications due to their controllability and versatility. Despite their significance, the realization and in-depth characterization of ferromagnetic materials in atomically thin single layers, close to the true 2D limit, has been scarce. Here, a successful synthesis of monolayer (ML) 1T-CrTe is reported on a bilayer graphene (BLG) substrate via molecular beam epitaxy.
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September 2025
Department of Materials Science, Chiba University, 1-33 Yayoi-cho, Inage-ku, Chiba, 263-8522, Japan.
1D electronic structures on 2D crystalline surfaces are crucial for investigating low-dimensional quantum phenomena and enabling the development of dimensionally engineered nanodevices. However, the inherent periodic symmetry of 2D atomic lattices generally leads to delocalized electronic band extending across the surface, making the creation of periodic 1D electronic states a significant challenge. Here, robust 1D electronic ordering is demonstrated in ultrathin Mn films grown on an atomically flat, non-reconstructed body-centered cubic Fe substrate.
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September 2025
Department of Chemistry, Indian Institute of Technology, Kanpur, Uttar Pradesh, 208016, India.
Redox-active organic-inorganic hybrid electrode materials are promising candidates for eco-friendly, high-energy-density supercapacitors. The synergy between organic and inorganic components in energy storage devices has attracted considerable interest due to their complementary attributes, including flexibility, long-term stability, and high conductivity. This study presents an innovative approach for synthesizing an organic-inorganic active electrode material by grafting diazonium salts of 8-aminoquinoline (8-AQ-N ) onto CuFeO nanoparticle (NP) surfaces.
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