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Article Abstract
Combining electron and energy transfer processes is very significant for efficient photocatalytic oxidation of organic molecules. The first synthesized MOF, Co(L)(2,6-NDC)·guest (, L = bis(-pyridyl) tetrachloroperylene peryleneimide, 2,6-NDC = 2,6-naphthalenedicarboxylic acid, FJI = Fujian Institute), shows a 2-fold interpenetrated net, in which the 2,6-NDC ligand connects typical Co(COO) paddle wheel clusters to form square lattices pillared by new PDI-type ligand L. as a heterogeneous and recyclable photocatalyst is applied for photo-oxidation of benzylamine and its derivatives with an excellent yield of 100%, which is much higher than that (59%) of the equivalent L ligand as a homogeneous photocatalyst under the same reaction conditions. Such a high-efficiency photocatalytic activity attributes to the combination of charge and energy transfer processes in catalyst during the catalytic process.
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| http://dx.doi.org/10.1021/acs.inorgchem.9b03743 | DOI Listing |
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