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Article Abstract
Using synchrotron surface X-ray diffraction, we investigated the atomic structures of the interfaces of a solid electrolyte (LiPO) and electrode (LiCoO). We prepared two types of interfaces with high and low interface resistances; the low-resistance interface exhibited a flat and well-ordered atomic arrangement at the electrode surface, whereas the high-resistance interface showed a disordered interface. These results indicate that the crystallinity of LiCoO at the interface has a significant impact on interface resistance. Furthermore, we reveal that the migration of Li ions along the interface and into grain boundaries and antiphase domain boundaries is a critical factor reducing interface resistance.
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| http://dx.doi.org/10.1021/acsami.8b08926 | DOI Listing |
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