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We describe a robust system for laser-driven narrowband terahertz generation with high conversion efficiency in periodically poled Lithium Niobate (PPLN). In the multi-stage terahertz generation system, the pump pulse is recycled after each PPLN stage for further terahertz generation. By out-coupling the terahertz radiation generated in each stage, extra absorption is circumvented and effective interaction length is increased. The separation of the terahertz and optical pulses at each stage is accomplished by an appropriately designed out-coupler. To evaluate the proposed architecture, the governing 2-D coupled wave equations in a cylindrically symmetric geometry are numerically solved using the finite difference method. Compared to the 1-D calculation which cannot capture the self-focusing and diffraction effects, our 2-D numerical method captures the effects of difference frequency generation, self-phase modulation, self-focusing, beam diffraction, dispersion and terahertz absorption. We found that the terahertz generation efficiency can be greatly enhanced by compensating the dispersion of the pump pulse after each stage. With a two-stage system, we predict the generation of a 17.6 mJ terahertz pulse with total conversion efficiency η = 1.6% at 0.3 THz using a 1.1 J pump laser with a two-lines spectrum centered at 1 μm. The generation efficiency of each stage is above 0.8% with the out-coupling efficiencies above 93.0%.
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http://dx.doi.org/10.1364/OE.26.029744 | DOI Listing |
Phys Rev Lett
August 2025
University of Delaware, Department of Physics and Astronomy, Newark, Delaware 19716, USA.
Ultrafast light-driven strongly correlated antiferromagnetic insulators, such as prototypical NiO with a large Mott energy gap ≃4 eV, have recently attracted experimental attention using photons of both subgap [H. Qiu et al., Nat.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
University of Konstanz, Department of Physics and Center for Applied Photonics, D-78457 Konstanz, Germany.
Femtosecond laser excitation of nanometer thin heterostructures comprising a heavy metal and a magnetically ordered material is known to result in the emission of terahertz radiation. However, the nature of the emitted radiation from heavy metal/antiferromagnet heterostructures has sparked debates and controversies in the literature. Here, we unambiguously separate spin and charge contributions from Pt/NiO heterostructures by introducing an unprecedented methodology combining high external magnetic fields with a symmetry analysis of the emitted terahertz polarization.
View Article and Find Full Text PDFMicrosyst Nanoeng
September 2025
Center for Terahertz Waves, College of Precision Instrument and Optoelectronics Engineering, and the Key Laboratory of Optoelectronics Information and Technology (Ministry of Education), Tianjin University, Tianjin, 300072, China.
Terahertz communication systems demand versatile devices capable of simultaneously controlling propagating waves and surface plasmon polaritons (SPPs) in far-field (FF) and near-field (NF) channels, yet existing solutions are constrained by volatile operation, single-function limitations, and the inability to integrate NF and FF functionalities. Here, we present a nonvolatile reconfigurable terahertz metasurface platform leveraging the phase-change material GeSbTe(GST) to achieve on-demand dual-channel modulation-a first in the terahertz regime. By exploiting the stark conductivity contrast of GST between amorphous and crystalline states, our design enables energy-efficient switching between NF-SPP manipulation and FF-wavefront engineering without requiring continuous power input.
View Article and Find Full Text PDFACS Nano
September 2025
College of Physics, Donghua University, Shanghai 201620, China.
Broadband anisotropic photodetectors show great promise for polarization-sensitive imaging and multispectral optoelectronic systems yet face critical challenges in material anisotropy modulation and broadband sensitivity. Weyl semimetals exhibit giant optical anisotropy and tunable heterojunction band alignment, enabling high-performance anisotropic photodetection. Herein, ultrabroadband PDs based on the NbNiTe (niobium nickel telluride), enabled by antenna integration and heterostructure engineering, achieve high sensitivity from visible to Terahertz (THz).
View Article and Find Full Text PDFNano Lett
September 2025
Department of Mechanical Engineering, Pohang University of Science and Technology (POSTECH), Pohang, 37673, Republic of Korea.
Active manipulation of terahertz (THz) waves is important for future optoelectronic applications, but most approaches rely on volatile or slow actuation, limiting efficiency and stability. Here, we report a nonvolatile, low-voltage tunable THz transmission device based on electrochemical modulation of a conductive polymer thin film integrated with metallic nanoresonators. A thin film of PEDOT:PSS, deposited via a single-step spin-coating process onto the nanoresonator array, enables efficient modulation of resonance-enhanced THz transmission with a gate voltage of less than 1 V.
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