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Quantum interference lies at the foundation of many protocols for scalable quantum computing and communication with linear optics. To observe these effects the light source must emit photons that are indistinguishable. From a technological standpoint, it would be beneficial to have electrical control over the emission. Here we report of an electrically driven single-photon source emitting indistinguishable photons. The device consists of a layer of InAs quantum dots embedded in the intrinsic region of a p-i-n diode. Indistinguishability of consecutive photons is tested in a two-photon interference experiment under two modes of operation, continuous and pulsed current injection. We also present a complete theory based on the interference of photons with a Lorentzian spectrum which we compare to both our continuous wave and pulsed experiments. In the former case, a visibility was measured limited only by the timing resolution of our detection system. In the case of pulsed injection, we employ a two-pulse voltage sequence which suppresses multi-photon emission and allows us to carry out temporal filtering of photons which have undergone dephasing. The characteristic Hong-Ou-Mandel 'dip' is measured, resulting in a visibility of 64 +/- 4%.
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http://dx.doi.org/10.1088/0957-4484/21/27/274011 | DOI Listing |
J Chem Phys
September 2025
Key Laboratory of Materials Modification by Laser, Electron, and Ion Beams (Ministry of Education), School of Physics, Dalian University of Technology, Dalian 116024, People's Republic of China.
This study investigates the stereodynamical control of the H + HBr (v = 0, j = 1) reaction within 0.01-1.50 eV collision energy using the time-dependent wave packet method.
View Article and Find Full Text PDFNat Photonics
June 2025
University of Vienna, Faculty of Physics, Vienna Center for Quantum Science and Technology (VCQ), Vienna, Austria.
Recently, machine learning has had remarkable impact in scientific to everyday-life applications. However, complex tasks often require the consumption of unfeasible amounts of energy and computational power. Quantum computation may lower such requirements, although it is unclear whether enhancements are reachable with current technologies.
View Article and Find Full Text PDFAnal Chim Acta
November 2025
Guangxi Key Laboratory of Natural Polymer Chemistry and Physics, Key Laboratory of Nanobiosensor Analysis, College of Chemistry and Materials, Nanning Normal University, Nanning, 530001, PR China. Electronic address:
Background: Hexavalent chromium ions (Cr(VI)), a notorious toxic heavy metal pollutant with proven carcinogenicity, endangers human health and the environment. Meanwhile, l-ascorbic acid (L-AA), a vital biological antioxidant, has abnormal levels closely tied to various diseases. Developing efficient synchronous detection methods for these two key analytes is of great value in clinical and environmental monitoring.
View Article and Find Full Text PDFSpectrochim Acta A Mol Biomol Spectrosc
September 2025
Institute of Functional Molecules, Shenyang University of Chemical Technology, Shenyang 110142, China.
A new variety of nitrogen-doped carbon dots (NCDs) was produced using a hydrothermal synthesis method, based on propanedioic acid and barbituric acid as the sources of carbon and nitrogen. The NCDs were analyzed by X-ray photoelectron spectroscopy (XPS), transmission electron microscopy (TEM), Zeta Potential,X-ray Diffraction(XRD),Thermogravimetry-Derivative Thermogravimetry(TG-DTG),Fourier transform infrared spectroscopy (FTIR) and Fluorescence Lifetime. The characterization results indicate that NCDs possess an average diameter of approximately 2.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
September 2025
School of Chemistry, Faculty of Exact Sciences, Tel-Aviv University, Tel Aviv, 69978, Israel.
Chemiluminescence offers distinct advantages for bioimaging and sensing, notably by eliminating the need for external light excitation and minimizing background interference. While the original phenoxy-1,2-dioxetanes have served as the cornerstone of chemiluminescent probe design, their efficiency is significantly compromised in aqueous environments. In this study, we report the development and evaluation of phenylamine-substituted 1,2-dioxetanes as a new class of luminophores with markedly enhanced performance under physiological conditions.
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