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Article Abstract
0D hybrid manganese halides represent an emerging class of luminescent materials, yet their practical application has been hindered by the intrinsic trade-off between optical performance and mechanical flexibility. Here, a green synthesis of 0D (ECMP)MnBr crystal is reported, exhibiting unprecedented triple-mode emission (photoluminescence, X-ray scintillation, and mechanoluminescence) through rationally designed highly symmetric [MnBr] tetrahedra, achieving near-unity photoluminescence quantum yield (98.97%), record-low X-ray detection limit (15.62 nGy s) and multi-stimuli responsiveness (rubbing, squeezing, stretching). The material's ultralow electron-phonon coupling (S = 1.438) and defect-suppressing π-π stacking enable exceptional environmental stability and closed-loop recyclability via solvent-mediated recrystallization. Innovatively, (ECMP)MnBr is first integrated into thermoplastic polyurethane via wet-spinning, simultaneously retaining single-crystal emission intensity and achieving remarkable elasticity (>1000% strain) for deformation-resistant wearable applications. This work establishes a new design paradigm for sustainable multifunctional optoelectronics, with immediate applications in wearable displays, high-resolution X-ray imaging, and self-powered optical sensors.
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