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Electromagnetic resonant systems, such as cavities and LC circuits, are widely used to detect ultralight boson dark matter and high-frequency gravitational waves. However, the narrow bandwidth of single-mode resonators necessitates multiple scan steps to cover broad frequency ranges. By incorporating a network of auxiliary modes via beam-splitter-type and non-degenerate parametric couplings, we enable broadband detection with an effective bandwidth of each scan matching the order of the resonant frequency, while maintaining a strong signal response. In heterodyne upconversion detection, where a background cavity mode transitions into another due to a potential background source, multiple orders of the source frequency can be probed with high sensitivity without tuning the cavity frequency. Consequently, our method allows for significantly deeper exploration of the parameter space within the same integration time compared to single-mode detection.
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http://dx.doi.org/10.1088/1361-6633/add050 | DOI Listing |
J Chem Phys
September 2025
Department of Chemistry, Zhejiang University, Hangzhou, Zhejiang Province 310027, China.
Sum-frequency generation vibrational spectroscopy (SFG-VS) has been well-established as a unique spectroscopic probe to interrogate the structure, interaction, and dynamics of molecular interfaces, with sub-monolayer sensitivity and broad applications. Sub-1 cm-1 High-Resolution Broadband SFG-VS (HR-BB-SFG-VS) has shown advantages with high spectral resolution and accurate spectral line shape. However, due to the lower peak intensity for the long picosecond pulse used in achieving sub-wavenumber resolution in the HR-BB-SFG-VS measurement, only molecular interfaces with relatively strong signal have been studied.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
National Key Laboratory of Advanced Micro and Nano Manufacture Technology, Shanghai Jiao Tong University, Shanghai 200240, China.
Integrating surface-enhanced fluorescence (SEF) and surface-enhanced Raman spectroscopy (SERS) into a single probe is a natural step forward for plasmon-enhanced spectroscopy (PES), as SEF enables enhanced fluorescent imaging for fast screening of targets, while SERS allows ultrasensitive trace molecular characterization with specificity. However, many challenges remain, e.g.
View Article and Find Full Text PDFAdv Sci (Weinh)
September 2025
College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing, 211100, P. R. China.
Aircraft confronting harsh meteorological conditions and radar detection environments during high-altitude flights face significant risks, which can threaten flight safety. This study designs and fabricates a novel Jerusalem cross-inspired Frequency Selective Surface (FSS). Initially, rGO powder with an optimized reduction degree is synthesized as the conductive filler.
View Article and Find Full Text PDFJ Colloid Interface Sci
September 2025
College of Physics and Electronic Information, Yunnan Key Laboratory of Optoelectronic Information Technology, Yunnan Normal University, Kunming 650500, China. Electronic address:
Antimony trisulfide (SbS) has emerged as a promising inorganic semiconductor for optoelectronics due to its distinctive anisotropic crystal structure and suitable bandgap (∼1.7 eV). While hydrothermal synthesis remains challenging for achieving high crystallinity and controlled morphology, we developed an innovative dual‑sulfur precursor strategy utilizing sodium thiosulfate (STS) and thioacetamide (TAA) at a 7:2 M ratio with SbCl.
View Article and Find Full Text PDFLangmuir
September 2025
Materials and Manufacturing Directorate, Air Force Research Laboratory, Wright-Patterson AFB, Dayton, Ohio 45433, United States.
Aluminum nanoparticles (Al NPs) were synthesized via catalyzed thermal reduction of an aluminum precursor in the presence of a capping ligand. A systematic study was conducted to examine the effect of dilution on nanoparticle synthesis by varying the volume of anhydrous toluene across four dilution factors while maintaining constant molar quantities of the aluminum precursor, catalyst, and ligand. This methodology is relevant for scale-up processes, where more dilute conditions can mitigate nanoparticle reactivity and enhance safety.
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