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Article Abstract
The transformation of CO into value-added products from an impure CO stream, such as flue gas or exhaust gas, directly contributes to the principle of carbon capture and utilization (CCU). Thus, we have developed a robust iron-based heterogeneous photocatalyst that can convert the exhaust gas from the car into CO with an exceptional production rate of 145 μmol g h. We characterized this photocatalyst by PXRD, XPS, ssNMR, EXAFS, XANES, HR-TEM, and further provided mechanistic experiments, and multi-scale/level computational studies. We have reached a clear understanding of its properties and performance that indicates that this highly robust photocatalyst could be used to design an efficient visible-light-mediated reduction strategy for the transformation of impure CO streams into value-added products.
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| http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11268485 | PMC |
| http://dx.doi.org/10.1039/d4sc02773f | DOI Listing |
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