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The fermionic Hubbard model (FHM) describes a wide range of physical phenomena resulting from strong electron-electron correlations, including conjectured mechanisms for unconventional superconductivity. Resolving its low-temperature physics is, however, challenging theoretically or numerically. Ultracold fermions in optical lattices provide a clean and well-controlled platform offering a path to simulate the FHM. Doping the antiferromagnetic ground state of a FHM simulator at half-filling is expected to yield various exotic phases, including stripe order, pseudogap, and d-wave superfluid, offering valuable insights into high-temperature superconductivity. Although the observation of antiferromagnetic correlations over short and extended distances has been obtained, the antiferromagnetic phase has yet to be realized as it requires sufficiently low temperatures in a large and uniform quantum simulator. Here we report the observation of the antiferromagnetic phase transition in a three-dimensional fermionic Hubbard system comprising lithium-6 atoms in a uniform optical lattice with approximately 800,000 sites. When the interaction strength, temperature and doping concentration are finely tuned to approach their respective critical values, a sharp increase in the spin structure factor is observed. These observations can be well described by a power-law divergence, with a critical exponent of 1.396 from the Heisenberg universality class. At half-filling and with optimal interaction strength, the measured spin structure factor reaches 123(8), signifying the establishment of an antiferromagnetic phase. Our results provide opportunities for exploring the low-temperature phase diagram of the FHM.
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http://dx.doi.org/10.1038/s41586-024-07689-2 | DOI Listing |
J Am Chem Soc
September 2025
Department of Chemistry, Princeton University, Princeton, New Jersey 08544, United States.
Layered van der Waals (vdW) materials, characterized by their interlayer vdW gaps, offer exceptional tunability of magnetic properties via intercalation chemistry. A wide range of magnetic behaviors have been observed in nonmagnetic transition-metal dichalcogenides intercalated with magnetic atoms. Beyond the incorporation of magnetic ions, we propose the controlled alkali-ion intercalation of intrinsic vdW magnets as a strategy to probe and manipulate spin populations and exchange interactions within individual magnetic layers.
View Article and Find Full Text PDFInorg Chem
September 2025
Chemistry Department and Center for Material Science and Nanotechnology, University of Oslo, Oslo NO-0315, Norway.
The Jahn-Teller effect significantly affects the CrF octahedra in Cr(II) fluoroperovskites. Here, we report the synthesis, crystal structures, and magnetic properties of RbCrF and CsCrF, thereby completing a comprehensive investigation of the CrF fluoroperovskites. Powder samples are prepared using a wet-chemical method, which allows stabilization of Cr(II).
View Article and Find Full Text PDFJ Am Chem Soc
September 2025
Institute of Inorganic and Analytical Chemistry, University of Münster, Corrensstrasse 28/30, 48149 Münster, Germany.
Materials exhibiting coexisting exploitable properties often result in especially attractive behavior from both fundamental and applied perspectives. In particular, magnetoelectric materials combining ferroelectric and magnetic properties are increasingly becoming paramount nowadays. Here, we show that FeH(PO) exhibits proton conductivity and the coexistence of magnetic and polar structural features, suggesting that such frameworks may be of broader interest beyond the field of proton conductors.
View Article and Find Full Text PDFSmall
September 2025
Department of Materials Science, Chiba University, 1-33 Yayoi-cho, Inage-ku, Chiba, 263-8522, Japan.
1D electronic structures on 2D crystalline surfaces are crucial for investigating low-dimensional quantum phenomena and enabling the development of dimensionally engineered nanodevices. However, the inherent periodic symmetry of 2D atomic lattices generally leads to delocalized electronic band extending across the surface, making the creation of periodic 1D electronic states a significant challenge. Here, robust 1D electronic ordering is demonstrated in ultrathin Mn films grown on an atomically flat, non-reconstructed body-centered cubic Fe substrate.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
Department of Physics, University of Sargodha, 40100 Sargodha, Pakistan.
The BaGdRuO double perovskite oxide demonstrates intriguing behavior, arising from competing antiferromagnetic (AFM) and ferrimagnetic (FiM) phases. Under the GGA++SOC scheme, the system exhibits an AFM ground state with a very small energy difference of -11.39 meV compared to the FiM one.
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