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A tower air filtration system was designed in which bead air filters (BAFs) were actively rotated by a fan motor to remove particulate matter (PM) or HCHO gas. Three types of BAF, hydrophilic, hydrophobic, and hybrid, were prepared and compared for the removal of PM and HCHO gas. A tower air filtration system loaded with hybrid BAFs purified 3.73 L of PM (2500 μg/m PM) at a high flow rate of 3.4 m/s with high removal efficiency (99.4% for PM) and a low pressure drop (19 Pa) in 6 min. Against our expectations, the PM removal efficiency slightly increased as the air velocity increased. The hybrid BAF-200 showed excellent recyclability up to 50 cycles with high removal efficiencies (99.4-93.4% for PM). Furthermore, hydrophilic BAF-200 could permanently remove 3.73 L of HCHO gas (4.87 ppm) and return the atmosphere to safe levels (0.41-0.31 ppm) within 60 min without any desorption of HCHO gas.
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http://dx.doi.org/10.3390/polym14030422 | DOI Listing |
Toxics
July 2025
Key Laboratory for Urban Habitat Environmental Science and Technology, Peking University Shenzhen Graduate School, Shenzhen 518055, China.
Understanding the differential impacts of emission sources of volatile organic compounds (VOCs) on formaldehyde (HCHO) levels is pivotal to effectively mitigating key photochemical radical precursors, thereby enhancing the regulation of atmospheric oxidation capacity (AOC) and ozone formation. This investigation systematically selected and analyzed year-long VOC measurements across three urban zones in Shenzhen, China. Photochemical age correction methods were implemented to develop the initial concentrations of VOCs before source apportionment; then Positive Matrix Factorization (PMF) modeling resolved six primary sources: solvent usage (28.
View Article and Find Full Text PDFACS EST Air
August 2025
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, Georgia 30332, United States.
Missing sulfate production pathways have been implicated as the cause of model underestimates of sulfate during haze events in East Asia. We add multiphase oxidation of SO in aerosol particles by HO, O, NO, HCHO, and O, catalyzed by transition metal ions (TMIs), to the GEOS-Chem model and evaluate the model with (1) year-round ground-based observations in Seoul, South Korea, (2) airborne observations from the KORUS-AQ field campaign, and (3) fall and winter ground-based observations in Beijing, China. Multiphase chemistry contributes 14% to 90% to total sulfate production depending on the location and season and increases model daily average sulfate by 2 to 3 μg m, with maximum daily increases up to 12 μg m.
View Article and Find Full Text PDFNat Commun
August 2025
State Key Laboratory of Advanced Fiber Materials, College of Materials Science and Engineering, Institute of Functional Materials, Donghua University, Shanghai, China.
The partial oxidation of methane (POM) into value-added C chemicals (e.g., CHOH, HCHO, and CO) offers a promising approach for natural gas utilization under mild conditions.
View Article and Find Full Text PDFACS Sens
August 2025
School of Physics and Optoelectronics & Hunan Institute of Advanced Sensing and Information Technology, Xiangtan University, Xiangtan 411105, PR China.
Indoor air pollution poses a major global health threat, with complex chemical components and low detection standards being core issues. Due to intrinsic cross-sensitivity, a wide range of commonly used resistive gas sensors struggle to accurately identify multiple gases in mixtures. Simultaneously identifying gas species and their concentrations has been a significant challenge in the field of gas detection.
View Article and Find Full Text PDFEnviron Sci Technol
August 2025
Joint International Research Laboratory of Atmospheric and Earth System Sciences, School of Atmospheric Sciences, Nanjing University, Nanjing 210023, China.
Hydroxymethanesulfonate (HMS) is an important reservoir of particulate sulfur, especially during winter haze episodes. However, the kinetics and mechanisms of HMS formation in aqueous aerosols remain poorly understood. In this study, we investigated the kinetics of the multiphase reaction between sulfur dioxide (SO) and formaldehyde (HCHO) in aqueous ammonium nitrate aerosol particles buffered by gas-phase NH at pH of 4.
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