Rare earth elements (REEs) are currently considered as contaminants of emerging concern, but their residual levels and trophic transfer in aquatic species and potential health risks are not fully characterized. This study compared the distribution patterns and trophodynamics of 15 REEs in the wild species of the Yellow River and adjacent Laizhou Bay of northern China. The daily intake of REEs through consuming aquatic products for Chinese residents was also estimated.
View Article and Find Full Text PDFThe ubiquitous and adverse effects of estrogens have aroused global concerns. Natural and synthetic estrogens in 255 water samples from the southern Bohai Sea were analyzed over three years. Total estrogen concentrations were 11.
View Article and Find Full Text PDFThe trophodynamic of organophosphate esters (OPEs) has not been known well despite their widespread occurrence in the aquatic environments. In this study, ten species of crustacean, seven species of mollusk, and 22 species of fish were collected in the Laizhou Bay (LZB) to examine the occurrence, bioaccumulation, and trophic transfer, and health risk of eight traditional OPEs and three emerging oligomeric OPEs. The results showed that total concentration of OPEs was 2.
View Article and Find Full Text PDFSewage treatment plants (STPs) are primary sources of antibiotics in aquatic environments. However, limited research has been conducted on antibiotic attenuation in STPs and their downstream waters in low-urbanized areas. This study analyzed 15 antibiotics in the STP sewage and river water in the Zijiang River basin to quantify antibiotic transport and attenuation in the STPs and downstream.
View Article and Find Full Text PDFThis study firstly investigated the effects of season, land use, and socioeconomic on the spatiotemporal changes of riverine antibiotic concentrations in a low urbanized and rural watershed. In the dry and wet seasons, water samples were collected and analyzed for 15 antibiotics. The results indicated that 14 antibiotics, excluding leucomycin, were detected.
View Article and Find Full Text PDFOrganophosphate esters (OPEs) are a group of synthetic chemicals used in numerous consumer products such as plastics and furniture. The Coronavirus Disease 2019 (COVID-19) pandemic significantly slowed anthropogenic activities and reduced the emissions of pollutants. Meanwhile, the mismanagement of large quantities of disposable plastic facemasks intensified the problems of plastic pollution and leachable pollutants in coastal waters.
View Article and Find Full Text PDFPharmaceuticals and personal care products (PPCPs) have captured global concern due to their detrimental effects on aquatic organisms. Thirty PPCPs were analyzed in the water of the Jiaozhou Bay watershed, the Yellow Sea (YS) and the East China Sea (ECS) in China to investigate the distribution and risk of PPCPs from rivers to coastal seas, which are not yet well documented. The results showed the prevalence of the target PPCPs with a downward trend in detection frequencies and total concentrations from rivers (675 ng/L on average) to bay (166 ng/L) and to coastal seas (103 ng/L).
View Article and Find Full Text PDFRecent studies have suggested that rare earth elements (REEs) are contaminants of emerging concern. Moreover, the understanding of the occurrence and risks of REEs in river-estuary-bay systems is limited. The present study investigated the distributions, geochemical characteristics, and ecological risks of Y and 14 REEs (La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, and Lu) in sediments from the Yellow River to its estuary and adjacent Laizhou Bay.
View Article and Find Full Text PDFGlobally, organophosphate esters (OPEs) have attracted substantial attention because of their ubiquity in the environment, toxicity, and potential ecological and health risks. This study comprehensively investigated the occurrence, partitioning, and spatial distribution of nine ordinary monomeric OPEs (m-OPEs) and three emerging oligomeric OPEs (o-OPEs) in a major tributary of the middle Yangtze River, which is the Zijiang River (ZR), and their associated potential health risks. Total OPE concentrations ranged from 18.
View Article and Find Full Text PDFMar Pollut Bull
February 2022
To investigate the long-term effects of urbanization and industrialization on coastal trace metal contamination, two sediment cores, Q21 (representing 1965-2018) and Q23 (representing 1986-2018), collected from the adjacent coasts of the east old town and west new area of Qingdao were analyzed. Although the concentrations of As, Cd, Co, Cr, Cu, Ni, Pb, Sc, and Zn were higher in Core Q21, the increasing trends in their concentrations and contamination levels were more obvious in Q23, especially since the 2000s. Moreover, the urbanization rates of the new area (1978-2017) were significantly positively correlated with the historical metal concentrations in Q23.
View Article and Find Full Text PDFThe concentrations, sources, and ecological risks of nine trace elements in nine rivers flowing into Laizhou Bay were investigated. The dissolved element concentrations were 1.85-74.
View Article and Find Full Text PDFOrganophosphate ester (OPE) levels, profiles, sources, spatial distribution, and partitioning were firstly studied in the rivers of the Shandong Peninsula. A total of 53 water samples and 45 sediment samples were collected from the rivers and the sewage treatment plant in the peninsula to quantitate levels of 13 targeted OPEs. Total OPE concentrations ranged from 263 to 6676 ng L in the water, and 39.
View Article and Find Full Text PDFHousehold and personal care products (HPCPs) are a kind of contaminants closely related to daily life, capturing worldwide concern. To our knowledge, this is the first attempt focusing on the spatiotemporal occurrence and mixture risk of HPCPs in the waters from rivers to Laizhou Bay. Nine HPCPs were quantitated in 216 water samples gathered from Laizhou Bay and its adjacent rivers in 2018, 2019, and 2021 to reveal the spatiotemporal occurrence and mixture ecological risks in Laizhou Bay.
View Article and Find Full Text PDFHeavy metal (HM) pollution in coastal ecosystems have posed threats to organisms and human worldwide. This study comprehensively investigated the concentrations, sources, trophodynamics, contamination, and risks of six HMs in the coastal ecosystem of Jiaozhou Bay, northern China, by stable isotope analysis, positive matrix factorization (PMF), and Monte Carlo simulation. Overall, Co, Cu, Ni, Pb, and Zn were significantly bio-diluted in the food web, while Cr was significantly biomagnified with a trophic magnification factor of 1.
View Article and Find Full Text PDFWe investigated the spatiotemporal distributions, risks, and prioritization of 15 widely used antibiotics in Laizhou Bay (LZB). Water samples (145) were collected from LZB and its estuaries and analyzed. Twelve antibiotics, with total concentrations of 241-1450 and 69-289 ng L in estuarine water and seawater, respectively, were detected, with the contributions of norfloxacin, ciprofloxacin, and amoxicillin exceeding 70%.
View Article and Find Full Text PDFLimited information is available on the spatiotemporal occurrence and ecological risks of organophosphate esters (OPEs) in coastal environments. 175 water samples were collected in Laizhou Bay (LZB) and its rivers and estuaries during spring and summer for the determination of 12 targeted OPEs. Total concentration of OPEs ranged from 234.
View Article and Find Full Text PDFArsenic (As) and antimony (Sb) are toxic metalloids widely distributed in coastal sediments, but are seldom studied for their geochemical baselines. In this study, sediment samples were collected from Jiaozhou Bay (JZB) to evaluate their baselines, contamination, and ecological risk. Results showed that the As and Sb concentrations were between 3.
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