Soil, food, and clean water are essential resources for sustaining human society and preserving ecological balance. However, the growing challenges of soil salinization and freshwater scarcity increasingly threaten global agricultural productivity and environmental health. This work presents an innovative Wash-Evaporate-Irrigate (WEI) system that integrates saline soil remediation, solar-powered freshwater recovery, salt resource harvest, and agricultural irrigation into a cohesive and sustainable process.
View Article and Find Full Text PDFChemosphere
February 2025
Cyanobacterial blooms are prevalent globally and present a significant threat to water security. Titanium salt coagulants have garnered considerable attention due to their superior coagulation properties and the absence of metal residue risks. This paper explored the influencing factors in the coagulation process of titanium xerogel coagulant (TXC), the alterations in cell activity during floc storage, and the release of cyanobacterial organic matters, thereby determining the application scope of TXC for cyanobacterial water treatment.
View Article and Find Full Text PDFFHWSB as an integrated absorptive catalyst, based on Walnut shell biochar (WSB) via hydrochloric acid modification and ferrous chloride impregnation, was prepared, reacted with HO to generate active free radicals •OH and •O, which oxidized and degraded about 80% of micro-pollutant sulfamethoxazole (SMX) from water, effectively resolving micro-pollutants' removal being inefficient because of high toxicity, persistence, and bioaccumulation in existed methods. It was clarified the specific degradation pathways and mechanisms of SMX by FHWSB synergistic HO via characterization and analysis assisted DFT calculations. Furthermore, it was found that the toxicity of a series of intermediates produced by SMX degraded continued to decline, consistent with its direction of degradation via toxicological analysis.
View Article and Find Full Text PDFActivated persulfate and hydrothermal treatment (HTT) are often employed to treat waste activated sludge, which can improve the efficiency of subsequent sludge treatment and change the distribution of pollutants in the sludge. However, the impact of sludge solid content and temperature on the occurrence and aging of microplastics (MPs) during HTT remains poorly understood. This study investigated the effects of persulfate-HTT (SPS-HTT) co-treatment on the migration, occurrence, and aging of MPs in sludge with different solid contents (2% and 5% solid content).
View Article and Find Full Text PDFWater Environ Res
March 2024
Eutrophication, the over-enrichment with nutrients, for example, nitrogen and phosphorus, of ponds, reservoirs and lakes, is an urgent water quality issue. The most notorious symptom of eutrophication is a massive proliferation of cyanobacteria, which cause aquatic organism death, impair ecosystem and harm human health. The method considered to be most effective to counteract eutrophication is to reduce external nutrient inputs.
View Article and Find Full Text PDFThe potential for the presence of microplastics (MPs) in municipal solid waste incineration bottom ash (MSWI-BA) has not been fully explored. In this study, surfactant-assisted air flotation separation in aqueous media was used to examine the removal of MPs and other pollutants from different particle size fractions of MSWI-BA. The use of 1 mmol L sodium dodecylbenzene sulfonate (SDBS), at a liquid-solid ratio of 60:1, increased by 66 % the quantity of MPs floated from the MSWI-BA 0-0.
View Article and Find Full Text PDFEnviron Technol
June 2024
Soil heavy metal pollution poses a serious threat to the eco-environment. Municipal sludge-based passivators and clay minerals have been widely applied to immobilize heavy metal contamination in soils. However, little is known about the immobilization effect and mechanisms of raw municipal sludge and clay in reducing the mobility and bioavailability of heavy metals in soils.
View Article and Find Full Text PDFWater Environ Res
March 2023
Due to the increasing use of antibiotics, tetracycline was frequently detected in wastewater. As a novel technology, algal-bacterial granular sludge process is expected to be widely used in wastewater treatment. However, the degradation effect of tetracycline by algal-bacterial granular sludge process and its degradation path is still unknown.
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February 2023
The immobilization of heavy metal pollutants in river and lake sediments is critical for environmental health and safety. In this study, combined electrokinetic and chemical immobilization were used to remediate Cd and Pb polluted river sediments. The effect of the concentrations of the immobilization reagents and the applied voltage were investigated.
View Article and Find Full Text PDFSci Total Environ
January 2023
Waste activated sludge and food waste are two typical important domestic low-value organic solid wastes (LOSW). LOSW contains significant organic matter and water content resulting in the transboundary transfer of liquid-solid-gas and other multi-mediums, such that the complexity of microplastics (MPs) migration should be of greater concern. This article provides a review of the literature focusing on the separation and extraction methods of MPs from LOSW.
View Article and Find Full Text PDFSci Total Environ
September 2022
Sewage treatment plants act as both sinks and sources of microplastics with elevated concentrations of microplastics accumulating in the sludge. Consequently, the effects of sludge conditioning and dewatering processes on the fate of microplastics need to be clarified. Microplastic characteristics in sludge, before and after advanced oxidation Fe(II)-activated persulfate conditioning were studied using a microplastics dynamic flotation separator (MDFS).
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
August 2022
Microplastics are frequently detected in wastewater treatment plants, but the knowledge of their effects on microalgal-bacterial granular sludge (MBGS) is still unknown. This study investigated the performance and adaptive response of MBGS exposed in municipal wastewater in the presence of polystyrene (PS) microplastic particles with different sizes (i.e.
View Article and Find Full Text PDFWater Environ Res
December 2021
Heavy metals and metalloids, in sludge and sediments, are environmental pollutants of concern with long-term negative effects on human and ecological health. In this study, sludge from biological treatment of municipal waste leachate was pyrolyzed into leachate sludge-derived biochar (LSDB) at 300°C to 900°C, comprising complex organic and inorganic (particularly heavy metals) species formed from heterogeneous chemical reactions. Based on different advanced material analyses, that is, Thermogravimetric Analysis (TGA), Fourier transform infrared (FTIR), scanning electron microscopy (SEM), and X-ray diffraction (XRD) analysis, this study revealed that mass loss and microstructural changes of LSDBs occurred primarily due to decomposition of volatiles, aromatic rings, carbonates, and hydroxides.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
February 2022
Sludge conditioning is important for improved dewatering, with the sludge characteristics impacting the effect of conditioning. A composite conditioner, Fe-activated sodium persulfate (Fe/SPS) combined with phosphogypsum (PG), was used to examine its impact on sludges with different organic contents (34.6-43.
View Article and Find Full Text PDFDisposal of dredged river sediment requires decreases in both water content for reduction in disposal area, and the amount of eutrophication pollutants at risking of leaching. The effects of CaCl, polyferric sulfate (PFS) and calcified polyferric sulfate (CaPFS) on dewatering and phosphorus immobilization were examined. Upon CaPFS dosage of 1.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
August 2020
Artificial top-to-bottom water transmitting channels made of threads of wool blend (WT), cotton (CT), flax (FT), and polyethylene (PET) were used to enhance the dewater efficiency for river sediment. In addition, the disordered channels composed of 3-mm-long WT segments mixed randomly into the river sediment were also employed. The most effective dewatering channels were found to be top-to-bottom WT channels with water absorption capacity of 8.
View Article and Find Full Text PDFEnviron Pollut
August 2020
Chemical conditioning is an effective strategy for improved river sediment dewatering affecting both the dewatering efficiency and subsequent resource utilization of the dewatered cake. Two types of conditioning agents, polyaluminium chloride (PAC)/cationic polyacrylamide (PAM) (coagulation precipitation conditioning agent, referred to as P-P conditioning) and ferrous activated sodium persulfate (advanced oxidation conditioning agent, referred to as F-S conditioning) were examined. With increasing leach liquid to solid (L/S) ratio the concentration of Cd for the real time leachates from the dewatered cakes decreased, but the leaching ratio of Cd in both P-P and F-S dewatered cakes increased.
View Article and Find Full Text PDFElectro-dewatering (EDW) is an emerging technology for improved sludge/sediment dewatering enabling subsequent cost effective treatment for toxicity and pathogenic reduction if required and/or disposal, but the effects of sediment/sludge properties on the efficacy of EDW remain unclear. Here we investigate EDW in the absence of chemical conditioning which can result in secondary pollution. The influence of sediment/sludge volatile solids content (VS), electrical conductivity (EC), pH and zeta potential (ζ), on mechanical and electrical behaviors determining dewaterability and energy consumption (P) was investigated.
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March 2020
Traditional water treatment plants adopt multiple treatments to sequentially treat raw water for producing potable water. Besides complex treatment design and operation, they typically require a large space to accommodate different reactors. Furthermore, emerging issues (e.
View Article and Find Full Text PDFSci Total Environ
January 2019
A series of electro-dewatering experiments were conducted to explore the effect of sediment cake thickness (1-5 cm) and electric field strength (2-50 V cm). The final dry solids content, energy consumption and dewatering productivity were modeled and the validity of the model was tested. It was demonstrated that the electric field strength determines final dry solids content and the power utilization is an exponential function of electric field strength.
View Article and Find Full Text PDFWater Sci Technol
November 2017