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Riverine dissolved carbon (DC) plays a crucial role in global carbon cycle. Yet, the contribution of wastewater to global riverine DC remains unquantified. Here, we quantify the impact of treated and untreated domestic wastewater on dissolved inorganic carbon (DIC) and dissolved organic carbon (DOC) loadings at nation and river basin scales. We show that, globally, domestic wastewater discharges ~21.4 Tg DC annually-6.42 Tg DIC and 1.17 Tg DOC from treated, and 9.64 Tg DIC and 4.21 Tg DOC from untreated, collectively accounting for 3.13 ± 0.46% of the global riverine DC export. Contributions are highest in densely populated regions with high treatment capacity. Effluent DC levels are influenced by treatment technology, temperature, precipitation, economic growth and urban development. This underscores a need to incorporate the wastewater derived carbon into global carbon budget assessment, as well as to monitor and reduce carbon in wastewater effluents.
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http://dx.doi.org/10.1038/s41467-025-62920-6 | DOI Listing |
Nanoscale Adv
August 2025
Department of Metallurgical and Materials Engineering, Faculty of Engineering, University of Dokuz Eylül İzmir Turkey.
Thin films of CuSn Gd S were prepared on soda-lime glass substrates using spin coating in a sulfur-rich environment. We investigated how doping CuSnS with gadolinium (Gd) affected its structural, morphological, and optical properties using X-ray diffraction (XRD), Raman spectroscopy, field emission scanning electron microscopy (FE-SEM), and UV-Vis spectroscopy. XRD showed that all samples had a polycrystalline monoclinic structure, while FE-SEM revealed a mix of spherical and polygon-shaped grains.
View Article and Find Full Text PDFWater Res
August 2025
State Key Laboratory of Environmental Aquatic Chemistry, Key Laboratory of Drinking Water Science and Technology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.
Phosphorus is recognized as a major pollutant in municipal and domestic wastewater, but the effective removal of organic phosphorus (OP) using conventional wastewater treatment technologies is difficult. Herein, a novel visible light-enhanced Ti electrocoagulation (EC) technology was proposed for the removal of OP using 2-amino-ethyl phosphonic acid (AEP) as a model compound to elucidate the removal efficiency and mechanisms. The results showed that the irradiation under visible light (670 Lux) effectively enhanced the removal of AEP by Ti EC.
View Article and Find Full Text PDFOrganophosphate triesters (tri-OPEs) are synthetic phosphate derivatives that are primarily used as flame retardants and plasticizers. Tri-OPEs have become significant aquatic contaminants owing to their large production volumes and wide range of applications. Organophosphate diesters (di-OPEs) are closely related to tri-OPEs.
View Article and Find Full Text PDFSci Rep
September 2025
Petrolum Applications Department, Egyptian Petroleum Research Institute (EPRI), Ahmed El-Zomer, Nasr City, Cairo, Egypt.
An innovative composite membrane was developed by combining polyvinylidene fluoride (PVDF) with graphene oxide (GO), titania (TiO), and silica (SiO) nanoparticles (PGTS). This innovative membrane was created using solution casting and electrospinning techniques to enhance its surface area and hydrophilic characteristics, while incorporating photocatalytic properties for light-induced oil decomposition. The membrane structure was examined by scanning electron microscopy (SEM), X-ray diffraction (XRD), and Fourier transform infrared spectroscopy (FT-IR).
View Article and Find Full Text PDFEnviron Sci Technol
September 2025
Department of Civil and Environmental Engineering, Western University, London, Ontario N6A 3K7, Canada.
This study provides new field-based evidence of the physical and socioeconomic watershed factors and streamflow conditions that influence effluent inputs to streams from onsite wastewater treatment systems (OWTSs), including potential differences between inputs via slow (groundwater) and more rapid (subsurface preferential, overland, direct pipe) transport pathways. Stream sampling data were compiled for 46 watersheds in Ontario, Canada, with analyses including a conservative chemical tracer (acesulfame) representing all (slow and rapid) pathways and a nonconservative human fecal bacteria tracer (HF183) representing only rapid pathways. Acesulfame stream concentrations ranged from tens to over 1000 ng/L, indicating OWTS effluent inputs to streams are widespread.
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