Quantum spin liquid from electron-phonon coupling.

Proc Natl Acad Sci U S A

Institute for Advanced Study, Tsinghua University, Beijing 100084, China.

Published: August 2025


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Article Abstract

A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "nonengineered" microscopic model (or in any material) remains challenging. Here, using numerically exact sign-problem-free quantum Monte Carlo simulations, we show that a QSL arises in a nonengineered electron-phonon model. Specifically, we investigate the ground-state phase diagram of the bond Su-Schrieffer-Heeger model on a 2D triangular lattice at (one electron per site), which we show includes a QSL phase which is fully gapped, exhibits no symmetry-breaking order, and supports deconfined fractionalized holon excitations. This suggests promising routes for finding QSLs in realistic materials and high- superconductivity by lightly doping them.

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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC12377744PMC
http://dx.doi.org/10.1073/pnas.2426111122DOI Listing

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