A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "nonengineered" microscopic model (or in any material) remains challenging. Here, using numerically exact sign-problem-free quantum Monte Carlo simulations, we show that a QSL arises in a nonengineered electron-phonon model.
View Article and Find Full Text PDFBy explicit microscopic construction involving a mapping to a quantum vertex model subject to the "ice rule," we show that an electronically "trivial" band insulator with suitable vibrational (phonon) degrees of freedom can host a "resonating valence-bond" state-a quantum phase with emergent gauge fields. This type of band insulator is identifiable by the existence of emergent gapless "photon" modes and deconfined excitations, the latter of which carry nonquantized mobile charges. We suggest that such phases may exist in the quantum regimes of various nearly ferroelectric materials.
View Article and Find Full Text PDFInspired by the observation of increasingly one-dimensional (1D) behavior with decreasing temperature in small-angle twisted bilayers of WTe_{2} (tWTe_{2}), we theoretically explore the exotic sliding regimes that could be realized in tWTe_{2}. At zero displacement field, while hole-doped tWTe_{2} can be thought of as an array of weakly coupled conventional two-flavor 1D electron gases (1DEGs), the electron-doped regime is equivalent to coupled four-flavor 1DEGs, due to the presence of an additional "valley" degree of freedom. In the decoupled limit, the electron-doped system can thus realize phases with a range of interesting ordering tendencies, including 4k_{F} charge-density-wave and charge-4e superconductivity.
View Article and Find Full Text PDFWe image local superfluid density in single crystals of Pd-intercalated ErTe_{3} below the superconducting critical temperature T_{c}, well below the onset temperature T_{CDW} of (disordered) charge-density-wave order. We find no detectable inhomogeneities on micron scales. We observe a rapid increase of the superfluid density below T_{c}, deviating from the behavior expected in a conventional Bardeen-Cooper-Schrieffer superconductor, and show that the temperature dependence is qualitatively consistent with a combination of quantum and thermal phase fluctuations.
View Article and Find Full Text PDFThe two-dimensional electron gas is of fundamental importance in quantum many-body physics. We study a minimal extension of this model with C_{4} (as opposed to full rotational) symmetry and an electronic dispersion with two valleys with anisotropic effective masses. Electrons in our model interact via Coulomb repulsion, screened by distant metallic gates.
View Article and Find Full Text PDFWhen the electron-phonon coupling is quadratic in the phonon coordinates, electrons can pair to form bipolarons due to phonon zero-point fluctuations, a purely quantum effect. We study superconductivity originating from this pairing mechanism in a minimal model and reveal that, in the strong coupling regime, the critical temperature (T_{c}) is only mildly suppressed by the coupling strength, in stark contrast to the exponential suppression in linearly coupled systems, thus implying higher optimal T_{c} values. We demonstrate that large coupling constants of this flavor are achieved in known materials such as perovskites, and discuss strategies to realize such superconductivity using superlattices.
View Article and Find Full Text PDFSymmetry plays a key role in determining the physical properties of materials. By Neumann's principle, the properties of a material remain invariant under the symmetry operations of the space group to which the material belongs. Continuous phase transitions are associated with a spontaneous reduction in symmetry.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
November 2023
We study a simple electron-phonon model on square and triangular versions of the Lieb lattice using an asymptotically exact strong coupling analysis. At zero temperature and electron density n=1 (one electron per unit cell), for various ranges of parameters in the model, we exploit a mapping to the quantum dimer model to establish the existence of a spin-liquid phase with Z_{2} topological order (on the triangular lattice) and a multicritical line corresponding to a quantum critical spin liquid (on the square lattice). In the remaining part of the phase diagram, we find a host of charge-density-wave phases (valence-bond solids), a conventional s-wave superconducting phase, and with the addition of a small Hubbard U to tip the balance, a phonon-induced d-wave superconducting phase.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2023
Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is 1/ = 2, where is a dimensionless strength of the electron-phonon coupling. The fact that measured values satisfy ≲ 1 has been noted in the context of a possible "Planckian" bound on transport. However, since the electron-phonon scattering is quasielastic in this regime, no such Planckian considerations can be relevant.
View Article and Find Full Text PDFPhys Rev Lett
November 2022
The two-dimensional Wigner crystal (WC) occurs in the strongly interacting regime (r_{s}≫1) of the two-dimensional electron gas (2DEG). The magnetism of a pure WC is determined by tunneling processes that induce multispin ring-exchange interactions, resulting in fully polarized ferromagnetism for large enough r_{s}. Recently, Hossain et al.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
April 2022
Charge density waves (CDWs) have been observed in nearly all families of copper-oxide superconductors. But the behavior of these phases across different families has been perplexing. In La-based cuprates, the CDW wavevector is an increasing function of doping, exhibiting the so-called Yamada behavior, while in Y- and Bi-based materials the behavior is the opposite.
View Article and Find Full Text PDFUnidirectional ("stripe") charge density wave order has now been established as a ubiquitous feature in the phase diagram of the cuprate high-temperature superconductors, where it generally competes with superconductivity. Nonetheless, on theoretical grounds it has been conjectured that stripe order (or other forms of "optimal" inhomogeneity) may play an essential positive role in the mechanism of high-temperature superconductivity. Here, we report density matrix renormalization group studies of the Hubbard model on long four- and six-leg cylinders, where the hopping matrix elements transverse to the long direction are periodically modulated-mimicking the effect of putative period 2 stripe order.
View Article and Find Full Text PDFPhys Rev Lett
August 2021
Proc Natl Acad Sci U S A
September 2021
The elastocaloric effect (ECE) relates changes in entropy to changes in strain experienced by a material. As such, ECE measurements can provide valuable information about the entropy landscape proximate to strain-tuned phase transitions. For ordered states that break only point symmetries, bilinear coupling of the order parameter with strain implies that the ECE can also provide a window on fluctuations above the critical temperature and hence, in principle, can also provide a thermodynamic measure of the associated susceptibility.
View Article and Find Full Text PDFQuantum criticality may be essential to understanding a wide range of exotic electronic behavior; however, conclusive evidence of quantum critical fluctuations has been elusive in many materials of current interest. An expected characteristic feature of quantum criticality is power-law behavior of thermodynamic quantities as a function of a nonthermal tuning parameter close to the quantum critical point (QCP). Here, we observed power-law behavior of the critical temperature of the coupled nematic/structural phase transition as a function of uniaxial stress in a representative family of iron-based superconductors, providing direct evidence of quantum critical nematic fluctuations in this material.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2021
We analyze the quantum phase diagram of the Holstein-Hubbard model using an asymptotically exact strong coupling expansion. We find all sorts of interesting phases including a pair-density wave, a charge 4e (and even a charge 6e) superconductor, regimes of phase separation, and a variety of distinct charge-density-wave, spin-density-wave, and superconducting regimes. We chart the crossovers that occur as a function of the degree of retardation, i.
View Article and Find Full Text PDFIn the context of recent experimental observations of an unexpectedly large thermal Hall conductivity, κ_{H}, in insulating La_{2}CuO_{4} (LCO) and SrTiO_{3} (STO), we theoretically explore conditions under which acoustic phonons can give rise to such a large κ_{H}. Both the intrinsic and extrinsic contributions to κ_{H} are large in proportion to the dielectric constant, ε, and the "flexoelectric" coupling, F. While the intrinsic contribution is still orders of magnitude smaller than the observed effect, an extrinsic contribution proportional to the phonon mean-free path appears likely to account for the observations, at least in STO.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
December 2017
The paradigmatic example of a continuous quantum phase transition is the transverse field Ising ferromagnet. In contrast to classical critical systems, whose properties depend only on symmetry and the dimension of space, the nature of a quantum phase transition also depends on the dynamics. In the transverse field Ising model, the order parameter is not conserved, and increasing the transverse field enhances quantum fluctuations until they become strong enough to restore the symmetry of the ground state.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
May 2017
Using determinantal quantum Monte Carlo, we compute the properties of a lattice model with spin [Formula: see text] itinerant electrons tuned through a quantum phase transition to an Ising nematic phase. The nematic fluctuations induce superconductivity with a broad dome in the superconducting [Formula: see text] enclosing the nematic quantum critical point. For temperatures above [Formula: see text], we see strikingly non-Fermi liquid behavior, including a "nodal-antinodal dichotomy" reminiscent of that seen in several transition metal oxides.
View Article and Find Full Text PDFA key actor in the conventional theory of superconductivity is the induced interaction between electrons mediated by the exchange of virtual collective fluctuations (phonons in the case of conventional s-wave superconductors). Other collective modes that can play the same role, especially spin fluctuations, have been widely discussed in the context of high-temperature and heavy Fermion superconductors. The strength of such collective fluctuations is measured by the associated susceptibility.
View Article and Find Full Text PDFWe show that, measured in a backscattering geometry, the polar Kerr effect is absent if the nonlocal electromagnetic response function respects Onsager symmetry, characteristic of thermodynamic states that preserve time-reversal symmetry. A key element is an expression for the reflectivity tensor in terms of the retarded Green's function.
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