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Seeded free-electron lasers (FELs) capable of operating at repetition rates up to the MHz level are in high demand for advanced time-resolved spectroscopies, which require both full longitudinal coherence and high average photon flux in the extreme ultraviolet (EUV) and x-ray regimes. However, conventional external-seeding methods require ultraviolet seed lasers with peak powers on the order of 100 MW, constraining them to lower repetition rates. Here, we report the first lasing and stable operation of a direct-amplification enabled harmonic generation FEL driven by a weak seed laser with only MW-level peak power. Beginning with an ultraviolet seed laser with only 0.75 μJ pulse energy, we demonstrate its direct amplification to over 10 μJ within an 8-m-long modulator. We observe coherent harmonic generation up to the 12th harmonic of the seed and achieve saturation of the 7th harmonic in the radiator. These results represent a crucial milestone toward the realization of MHz-class, fully coherent EUV and x-ray light sources.
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http://dx.doi.org/10.1103/sslg-jjkz | DOI Listing |
J Chem Phys
September 2025
Jülich Centre for Neutron Science (JCNS-1), Forschungszentrum Jülich GmbH, 52428 Jülich, Germany.
The static and dynamic properties of a cyclic Rouse chain modified by the introduction of an effective, spherically symmetric, attracting potential of entropic nature are studied. It is shown that a relatively weak potential can lead to a strong contraction of the polymer chain: the radius of gyration becomes much smaller compared to the size of the free cyclic chain. The pronounced decrease in the terminal relaxation time of cyclic macromolecules in the presence of a harmonic potential compared to the Rouse relaxation time leads to a lengthening of the time interval for the transition to the normal, i.
View Article and Find Full Text PDFChem Sci
September 2025
State Key Laboratory of Crystal Materials, Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystals, Tianjin University of Technology Tianjin 300384 China
Nonlinear optical (NLO) crystals capable of expanding the spectral region of solid-state are of great importance for many high-tech applications, yet their rational structure design remains a great challenge because of the conflicting property requirements among second harmonic generation (SHG) response, ultraviolet (UV) cut-off edge, and birefringence. Herein, based on the chemical disubstitution of the classic NLO crystal SrBeBO (SBBO), , substituting [BO] triangles with larger π-conjugated [BO] groups and substituting high-toxic [BeO] tetrahedra with environment-friendly [AlO] tetrahedra, a new high-performance aluminoborate NLO crystal, BaAlBO, has been successfully designed and synthesized. The theoretical calculations and optical property measurements indicate that BaAlBO exhibits not only the largest SHG response among the reported aluminoborates (2.
View Article and Find Full Text PDFAdv Mater
September 2025
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environmental Conditions, Xinjiang Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Urumqi, 830011, P. R. China.
The generation of coherent deep-ultraviolet (DUV) radiation via nonlinear frequency conversion remains a major scientific and technological challenge in modern optics. To date, only a very limited number of nonlinear optical (NLO) crystals-such as KBBF, ABF, and quartz-have been experimentally demonstrated to support measurable direct second-harmonic generation (SHG) at wavelengths of 177 nm or shorter. There is a pressing need to develop alternative materials or strategies that enable efficient frequency conversion in the DUV region.
View Article and Find Full Text PDFThis paper presents a novel multiscale signal processing framework for power quality disturbance (PQD) and cyber intrusion detection in smart grids, combining Non-Subsampled Contourlet Transform (NSCT), Split Augmented Lagrangian Shrinkage Algorithm (SALSA), and Morphological Component Analysis (MCA). A key innovation lies in an adaptive weighting mechanism within NSCT's directional sub bands, enabling dynamic energy redistribution and enhanced representation of both low-frequency anomalies (e.g.
View Article and Find Full Text PDFCarbohydr Polym
November 2025
Molecular Imaging and Photonics, Department of Chemistry, KU Leuven, Campus Kulak Kortrijk, Etienne Sabbelaan 53, 8500 Kortrijk, Belgium. Electronic address:
Cellulose nanocrystals (CNCs) have emerged as promising candidates for chiroptical functional materials due to their ability to form cholesteric liquid crystals with tunable periodicity. The quality of the final cholesteric phase is influenced by the nucleation, growth and coalescence mechanism of the initial droplets, known as tactoids. Current research focuses on understanding the size and morphological transformations of these tactoids, to gain deeper insights into their dynamic behavior and, in turn, to better control the final properties of novel photonic materials.
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