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Article Abstract
High-Ni cathodes promise high energy density but suffer from interfacial degradation. Here, a dual-additive electrolyte-trimethylsilyl phosphate to scavenge HF and adiponitrile to tailor Li solvation-enables a robust, LiF-rich CEI, boosting NCM811's stability. This strategy achieves 90.16% capacity retention at 5C, offering a pathway to durable, high-performance batteries.
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| http://dx.doi.org/10.1039/d5cc01939g | DOI Listing |
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