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We present a novel method for generating spin currents using the gyromagnetic effect, a phenomenon discovered over a century ago. This effect, crucial for understanding the origins of magnetism, enables the coupling between various macroscopic rotational motions and electron spins. While higher rotational speeds intensify the effect, conventional mechanical rotations, typically, below 10,000 RPM, produce negligible results comparable to geomagnetic fluctuations, limiting applied research. Our studies demonstrate that spin current generation comparable to that of rare metals can be achieved through atomic rotations induced by GHz-range surface acoustic waves and the rotational motion of conduction electrons in metallic thin films with nanoscale gradient modulation of electrical conductivity. These effects, termed the acoustic gyromagnetic effect and the current-vorticity gyromagnetic effect, are significant in different contexts. The acoustic gyromagnetic effect is notable in high-conductivity materials like aluminum and copper, which are more abundant than conventional spintronics materials with strong spin-orbit interactions (SOIs). Conversely, the current-vorticity gyromagnetic effect requires a large conductivity gradient to produce current vorticity efficiently. This is achieved by using composition gradient structures from highly conductive metals to poorly conductive oxides or semiconductors. Consequently, unlike traditional strong-SOI materials, we can create highly efficient spin current generators with low energy dissipation due to reduced Joule loss.
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http://dx.doi.org/10.1080/14686996.2024.2428153 | DOI Listing |
Adv Mater
September 2025
College of Physics, Donghua University, Shanghai, 201620, China.
The 180° switching of the perpendicular Néel vector induced by the spin-orbit torque (SOT) presents significant potential for ultradense and ultrafast antiferromagnetic SOT-magnetoresistive random-access memory. However, its experimental realization remains a topic of intense debate. Here, unequivocal evidence is provided for the SOT-induced 180° switching of the perpendicular Néel vector in collinear antiferromagnetic CrO in a Pt/CrO/Co trilayer structure.
View Article and Find Full Text PDFIEEE Trans Med Imaging
September 2025
The T1rho mapping technique necessitates acquiring multiple T1rho-weighted images at various spin-lock times (TSL), which results in a lengthy scan time and significantly limits its widespread clinical use. Undersampling is a significant strategy to accelerate T1rho imaging, where it is crucial to model and utilize the joint spatiotemporal correlations priors among different TSL multi-contrast images for high-quality reconstruction. However, current methods that use simplified physical relaxation correlations or black-box deep neural networks to define joint correlations often yield inaccurate results.
View Article and Find Full Text PDFNano Lett
September 2025
School of Electrical Engineering, Southwest Jiaotong University, Chengdu 610032, People's Republic of China.
Precise modulation of the electronic structure in transition metals, particularly the d-band center position and spin state, remains a critical challenge to expediting hydrogen evolution reaction (HER) kinetics. Herein, we report a NiPt/Ni-heterostructured catalyst enabling simultaneous optimization of the d-band electronic structure and spin state of Ni through regulation of the NiPt and Ni bridge sites. Combining operando spectroscopy, X-ray absorption spectroscopy, density functional theory, and ab initio molecular dynamics simulations, we establish that the coordination environment and spin states of Ni at the bridge sites were effectively modulated by altering the Pt content, achieving a transition of Ni centers from the low-spin to high-spin state, and optimized intermediate adsorption/desorption behaviors.
View Article and Find Full Text PDFJ Am Chem Soc
September 2025
National Engineering Research Centre for Nanomedicine, College of Life Science and Technology, Huazhong University of Science and Technology, Wuhan 430074, P. R. China.
Image-guided surgery plays a critical role in improving the cancer patient prognosis. However, current clinical probes are often single-modal with "always-on" signals, failing to provide complementary and precise guidance across all perioperative phases. To tackle this hurdle, we develop a biomarker-activatable, multimodal nanoprobe - - based on redox-mediated manganese valence switching for tumor-specific, perioperative image-guided surgery.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
Department of Nanotechnology for Sustainable Energy, School of Science and Technology, Kwansei Gakuin University, 1 Gakuen-Uegahara, Sanda 669-1330, Japan.
Monolayer Janus transition-metal dichalcogenides possess Ising- and Rashba-type spin-orbit-couplings (SOC), leading to intriguing spin splitting effects at K and K', and around Γ points across the wide energy range. Using first-principles calculations, we unveil these SOC characteristics in metallic Janus NbSSe and demonstrate its potential for optically controlled spin current generation. On the basis of the symmetry of the system, we show that different linear polarized light can selectively drive spin currents of distinct spin components.
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