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In recent years, the rotational Doppler effect (RDE) has been widely used in rotational motion measurement. However, the performance of existing detection systems based on the RDE are generally limited by the drastic reduction of signal-to-noise ratio (SNR) due to the influence of atmospheric turbulence, partial obscuration of the vortex beam (VB) during propagation, and misalignment between the optical axis of VB and the rotational axis of the object, which poses a challenge for practical applications. In this paper, we proposed a coherent detection method of the RDE measurement based on triple Fourier transform. First, the weak RDE signal in backscattered light is amplified by using the balanced homodyne detection method, and the amplified signal still retains the same characteristic of severe broadening in the frequency domain as the original signal. Furthermore, we proposed the triple Fourier transform to extract the broadened RDE frequency shift signal after the coherent amplification. The proposed method significantly improves the SNR of RDE measurement and facilitates the accurate extraction of rotational speed, which helps to further improve the RDE detection range and promote its practical application.
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http://dx.doi.org/10.1364/OE.520674 | DOI Listing |
Inorg Chem
September 2025
School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, PR China.
Confronting the dual challenges of carbon neutrality and sustainable energy, photocatalytic CO reduction requires precise control over product selectivity. This study demonstrates that surface hydroxyl (-OH) density serves as a molecular switch for reaction pathways in graphene oxide/cobalt tetraphenylporphyrin (GO/CoTPP) hybrids. By tuning the reduction degree of GO supports via gradient hydrazine hydrate treatment (0-85%), we constructed catalysts with controlled -OH concentrations.
View Article and Find Full Text PDFJ Food Sci
September 2025
State Key Laboratory of Food Science and Resources, Jiangnan University, Wuxi, Jiangsu, China.
Numerous studies have been conducted on the interaction of β-lactoglobulin (β-LG) with catechins. However, the comparative discussion of multiple catechins interacting simultaneously with β-LG remains unknown. In this study, we comparatively investigated the interaction of three catechins with β-LG in various combinations, such as β-LG-EGCG ((-)-epigallocatechin gallate), β-LG-EGCG-EGC ((-)-epigallocatechin), and β-LG-EGCG-EGC-EC ((-)-epicatechin), and their underlying mechanisms through a series of spectroscopic analyses, molecular docking, and molecular dynamics simulations.
View Article and Find Full Text PDFIn Vivo
August 2025
Clinic and Policlinic for Dermatology and Venereology, University Medical Center Rostock, Rostock, Germany;
Background/aim: The aim of the present research is a comprehensive evaluation of a fish-collagen based wound membrane using established and methodologies. A porcine pericardium membrane served as control material.
Materials And Methods: Scanning electron microscopy (SEM) and attenuated total reflection-Fourier transform infrared spectroscopy (ATR-FTIR) analysis were initially used to analyze the structure and collagen molecular structure.
J Am Chem Soc
August 2025
State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, P. R. China.
Anthropogenic perfluoroalkyl and polyfluoroalkyl substances (PFAS) are pervasive contaminants subject to increasingly stringent regulatory thresholds in water resources. Current nonthermal defluorination strategies face critical limitations, including incomplete mineralization, yielding persistent short-chain PFAS byproducts, and residual fluoride ions, thereby hindering compliance with water quality standards. Herein, we demonstrate that wollastonite-bearing microdroplets prioritize defluorination over C-C scission in perfluoroalkyl chains through liquid-solid-gas triple-phase contact electrification.
View Article and Find Full Text PDFAnal Bioanal Chem
August 2025
Messina Institute of Technology, c/o Department of Chemical, Biological, Pharmaceutical and Environmental Sciences, former Veterinary School, University of Messina, Viale G. Palatucci snc 98168, Messina, Italy.
This research was focused on an in-depth investigation of 45 heroin samples seized in Northeast Italy, using complementary hyphenated analytical techniques. Gas chromatography coupled with mass spectrometry (GC-MS) and solid deposition Fourier transform infrared (FTIR) spectroscopy were employed to identify the seizure components. Common adulterants like caffeine and paracetamol were detected almost ubiquitously, along with other cutting agents from various chemical classes.
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