Colloidal quantum dot materials for next-generation near-infrared optoelectronics.

Chem Commun (Camb)

Department of Electrical and Computer Engineering, University of Alberta, Edmonton, Canada.

Published: January 2024


Category Ranking

98%

Total Visits

921

Avg Visit Duration

2 minutes

Citations

20

Article Abstract

Colloidal quantum dots (CQDs) are a promising class of materials for next-generation optoelectronic devices, such as displays, LEDs, lasers, photodetectors, and solar cells. CQDs can be obtained at low cost and in large quantities using wet chemistry. CQDs have also been produced using various materials, such as CdSe, InP, perovskites, PbS, PbSe, and InAs. Some of these CQD materials absorb and emit photons in the visible region, making them excellent candidates for displays and LEDs, while others interact with low-energy photons in the near-infrared (NIR) region and are intensively utilized in NIR lasers, NIR photodetectors, and solar cells. In this review, we have focused on NIR CQD materials and reviewed the development of CQD materials for solar cells, NIR lasers, and NIR photodetectors since the first set of reports on CQD materials in these particular applications.

Download full-text PDF

Source
http://dx.doi.org/10.1039/d3cc04315kDOI Listing

Publication Analysis

Top Keywords

cqd materials
16
solar cells
12
colloidal quantum
8
materials next-generation
8
displays leds
8
photodetectors solar
8
nir lasers
8
lasers nir
8
nir photodetectors
8
materials
7

Similar Publications

Precise control over the emission direction of colloidal quantum dots (CQDs), which are promising color conversion materials for micro-light-emitting-diode displays, is increasingly important for augmented-reality and virtual-reality near-eye optics. Here, we report a fully dielectric silicon nitride (SiN) photonic crystal (PhC) platform that boosts CQD photoluminescence by an 8.5-fold increase while compressing the angular full-width at half-maximum to 6.

View Article and Find Full Text PDF

Redefining PbS Quantum Dot Photovoltaics: p-i-n Devices with Superior Efficiency and Reproducibility.

Adv Mater

August 2025

Institute of Functional Nano & Soft Materials (FUNSOM), Joint International Research Laboratory of Carbon-Based Functional Materials and Devices, Soochow University, Suzhou, Jiangsu, 215123, PR China.

Developing diverse photovoltaic device architectures is essential not only for improving power conversion efficiency (PCE) but also for enabling seamless integration with other photovoltaic materials in high-performance tandem configurations. While n-i-p architectures have historically dominated the development of PbS colloidal quantum dots (CQDs) solar cells, p-i-n counterparts have significantly lagged behind in efficiency, limiting their potential for further advancement. In this work, the advantage of the surface tunability of CQDs is taken by anchoring the classical self-assembled monolayer (SAM) molecule MeO-2PACz onto PbS CQDs via ligand exchange, forming a PbS-SAM bridging-layer, which is inserted between NiOx/SAM and the CQD active layer, resulting in a NiOx/SAM/PbS-SAM composite hole transporting layer (HTL).

View Article and Find Full Text PDF

In dye-sensitized solar cells (DSSCs), the performance of commercially available TiO (P25, Degussa) is restricted by a low surface area and insufficient particle connectivity, resulting in hindered optoelectronic performance. This study presents an environmentally friendly and sustainable method for synthesizing TiO nanoparticles (NPs) using Sri Lankan ilmenite as a raw material. Additionally, carbon quantum dots (CQDs) are synthesized from coconut shells through a one-step hydrothermal carbonization process, providing a green synthesis process for these carbon-based nanomaterials.

View Article and Find Full Text PDF

PbS colloidal quantum dot photovoltaics: progress towards infrared and flexible applications.

Chem Commun (Camb)

August 2025

Department of Electrical and Computer Engineering, Johns Hopkins University, Baltimore, MD 21218, USA.

PbS colloidal quantum dots (CQDs) are a promising material class for near-infrared optoelectronics. The colloidal synthesis and fabrication pathways are readily scalable and compatible with a range of other materials and processes, and by controlling the size of the CQDs, the optical properties can be tuned over a wide spectral range in the visible and near-infrared (IR). This review article summarizes recent trends and advances in using PbS CQD devices for energy and photovoltaic applications.

View Article and Find Full Text PDF

Biomass-derived carbon quantum dots as fluorescent probes for biosensing: a review.

Chem Commun (Camb)

August 2025

State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology, Beijing, 100029, China.

The conversion of biomass waste into value-added carbon quantum dots (CQDs) has been recognized as a green synthetic pathway in CQD manufacturing. The distinctive nanostructure of biomass-derived carbon quantum dots (BCQDs) confers superior fluorescence properties and biocompatibility, rendering them highly promising as fluorescent probes for biosensing applications. The preparation of BCQD fluorescent probes using biomass as the primary carbon source not only realizes the high-quality recycling of waste resources but also has excellent biocompatibility and fluorescence emission stability, which has received great attention from researchers.

View Article and Find Full Text PDF