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Two-dimensional transition metal dichalcogenides (TMDCs) have properties attractive for optoelectronic and quantum applications. A crucial element for devices is the metal-semiconductor interface. However, high contact resistances have hindered progress. Quantum transport studies are scant as low-quality contacts are intractable at cryogenic temperatures. Here, temperature-dependent transfer length measurements are performed on chemical vapor deposition grown single-layer and bilayer WS devices with indium alloy contacts. The devices exhibit low contact resistances and Schottky barrier heights (∼10 kΩ μm at 3 K and 1.7 meV). Efficient carrier injection enables high carrier mobilities (∼190 cm V s) and observation of resonant tunnelling. Density functional theory calculations provide insights into quantum transport and properties of the WS-indium interface. Our results reveal significant advances toward high-performance WS devices using indium alloy contacts.
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http://dx.doi.org/10.1021/acsnano.0c05915 | DOI Listing |
Nature
September 2025
National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY, USA.
Controlling spin currents, that is, the flow of spin angular momentum, in small magnetic devices, is the principal objective of spin electronics, a main contender for future energy-efficient information technologies. A pure spin current has never been measured directly because the associated electric stray fields and/or shifts in the non-equilibrium spin-dependent distribution functions are too small for conventional experimental detection methods optimized for charge transport. Here we report that resonant inelastic X-ray scattering (RIXS) can bridge this gap by measuring the spin current carried by magnons-the quanta of the spin wave excitations of the magnetic order-in the presence of temperature gradients across a magnetic insulator.
View Article and Find Full Text PDFAnal Chem
September 2025
School of Agricultural Engineering, Key Laboratory of Modern Agricultural Equipment and Technology (Ministry of Education), Jiangsu University, Zhenjiang, Jiangsu 212013, PR China.
To balance the "detection sensitivity" and "device stability" of the organic photoelectrochemical transistor (OPECT) aptasensors, it has become an urgent challenge for achieving effective signal modulation under low ascorbic acid (AA) conditions. To address this, our work proposed a collaborative optimization strategy by coupling heterojunction engineering with interfacial molecular modulation, to endow a high current gain of OPECT with low-AA -dependence. First, a CdZnS-SnInS heterojunction gate was constructed by in situ growth of CdZnS quantum dots (QDs) on SnInS nanoflowers, which enhanced the light trapping ability and photoelectric conversion efficiency of the photoactive gate.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
Nanjing University, National Laboratory of Solid State Microstructures, Institute of Brain-Inspired Intelligence, School of Physics, Collaborative Innovation Center of Advanced Microstructures, Nanjing 210093, China.
The anomalous metal state (AMS), observed in "failed" superconductors, provides insights into superconductivity and quantum criticality, with studies revealing unconventional quantum phases like the Bose metal. Recently, layered transition metal dichalcogenide (TMD) superconductors approaching the two-dimensional limit have garnered significant attention for the enhanced phase fluctuations and electronic correlations. Investigating AMSs in these systems, particularly in the absence of an external magnetic field, could offer valuable insights into the dimensionality-driven emergence of exotic quantum phenomena, including triplet Cooper pairing, phase fluctuation dynamics, and especially the recently discovered field-free superconducting diode effects.
View Article and Find Full Text PDFJ Phys Chem Lett
September 2025
School of Materials Science and Engineering, Changchun University of Science and Technology, Changchun 130022, People's Republic of China.
Inverted quantum dot light-emitting diodes (QLEDs) show great promise for next-generation displays due to their compatibility with integrated circuit architectures. However, their development has been hindered by inefficient exciton utilization and charge transport imbalance. Here, we present a strategy for regulating charge-exciton dynamics through the rational design of a multifunctional hole transport layer (HTL), incorporating polyethylenimine ethoxylated (PEIE) as a protective interlayer in fully-solution-processed inverted red QLEDs.
View Article and Find Full Text PDFJ Phys Chem Lett
September 2025
Department of Chemistry and Chemical Biology, University of New Mexico, Albuquerque, New Mexico 87106, United States.
Defects significantly influence charge transport in CHNHPbI (MAPbI) perovskite solar cells, particularly at interfaces. Using quantum dynamics simulation, we reveal a distinct interstitial iodine (I) defect behavior at different positions in the TiO/MAPbI system. In the perovskite bulk-like region, I exhibits high mobility and dissociates detrimental iodine trimers, facilitating small-to-large polaron transition and promoting shallow trap formation.
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