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For realization the new functional materials and devices by conductive nanomaterials, how to control and realize the optimum network structures are import point for fundamental, applied and industrial science. In this manuscript, the nondestructive real-space imaging technique has been studied with the lock-in thermal scope via Joule heating caused by ac bias conditions. By this dynamical method, a few micrometer scale energy dissipations originating from local current density and resistance distributions are visualized in a few tens of minutes due to the frequency-space separation and the strong temperature damping of conductive heat components. Moreover, in the tensile test, the sample broken points were completely corresponding to the intensity images of lock-in thermography. These results indicated that the lock-in thermography is a powerful tool for inspecting the intrinsic network structures, which are difficult to observe by conventional imaging methods.
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http://dx.doi.org/10.1038/s41598-019-50802-z | DOI Listing |
J Synchrotron Radiat
May 2025
Center for Ultrafast Phase Transformation, Department of Physics, Sogang University, Seoul 04107, Republic of Korea.
Understanding atomic-level imperfections is crucial in various technological applications. Bragg coherent X-ray diffraction imaging (BCDI) enables non-destructive, three-dimensional imaging of those materials under in situ and operando conditions but has limited spatial resolution. This limitation hinders accurate calculations of physical quantities, e.
View Article and Find Full Text PDFAdv Sci (Weinh)
February 2024
School of Mechanical Engineering, Sungkyunkwan University (SKKU), Suwon-si, Gyeonggi-do, 16419, Republic of Korea.
Molecular electronics enables functional electronic behavior via single molecules or molecular self-assembled monolayers, providing versatile opportunities for hybrid molecular-scale electronic devices. Although various molecular junction structures are constructed to investigate charge transfer dynamics, significant challenges remain in terms of interfacial charging effects and far-field background signals, which dominantly block the optoelectrical observation of interfacial charge transfer dynamics. Here, tip-induced optoelectrical engineering is presented that synergistically correlates photo-induced force microscopy and Kelvin probe force microscopy to remotely control and probe the interfacial charge transfer dynamics with sub-10 nm spatial resolution.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
July 2023
Department of Materials Science and Engineering, Cornell University, Ithaca, NY 14853.
J Am Chem Soc
June 2023
Hefei National Research Center for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information & Quantum Physics, New Cornerstone Science Laboratory, University of Science and Technology of China, Hefei, Anhui 230026, China.
Isotope substitution of a molecule not only changes its vibrational frequencies but also changes its vibrational distributions in real-space. Quantitatively measuring the isotope effects inside a polyatomic molecule requires both energy and spatial resolutions at the single-bond level, which has been a long-lasting challenge in macroscopic techniques. By achieving ångström resolution in tip-enhanced Raman spectroscopy (TERS), we record the corresponding local vibrational modes of pentacene and its fully deuterated form, enabling us to identify and measure the isotope effect of each vibrational mode.
View Article and Find Full Text PDFSci Rep
January 2023
Division of Quantum Science and Engineering, Graduate School of Engineering, Hokkaido University, Kita-13 Nishi-8, Kita-ku, Sapporo, 060-8628, Japan.
Thermography using energy-dependent neutron transmission imaging can non-invasively and non-destructively visualize a real-space distribution of interior temperatures of a material in a container. Previously, resonance absorption broadening analysis and Bragg-edge shift analysis using energy-resolved neutron transmission have been developed, however some issues remain, e.g.
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