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In this study, segmented thermoelectric generators (TEGs) have been simulated with various state-of-the-art TE materials spanning a wide temperature range, from 300 K up to 1000 K. The results reveal that by combining the current best p-type TE materials, BiSbTe, MgAgSb, K-doped PbTeS and SnSe with the strongest n-type TE materials, Cu-Doped BiTeSe, AgPbSbTe and SiGe to build segmented legs, TE modules could achieve efficiencies of up to 17.0% and 20.9% at ΔT = 500 K and ΔT = 700 K, respectively, and a high output power densities of over 2.1 Watt cm(-2) at the temperature difference of 700 K. Moreover, we demonstrate that successful segmentation requires a smooth change of compatibility factor s from one end of the TEG leg to the other, even if s values of two ends differ by more than a factor of 2. The influence of the thermal radiation, electrical and thermal contact effects have also been studied. Although considered potentially detrimental to the TEG performance, these effects, if well-regulated, do not prevent segmentation of the current best TE materials from being a prospective way to construct high performance TEGs with greatly enhanced efficiency and output power density.
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http://dx.doi.org/10.1038/srep24123 | DOI Listing |
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September 2025
School of Materials Science and Engineering, Beihang University, Beijing, 100191, China.
Thermoelectric technology has significant applications in waste heat harvesting and temperature control of electronic devices. PbS has long been seen as a robust candidate for large-scale thermoelectric applications due to its low cost and high mechanical strength. However, the low ZT near room temperature hinders its further application.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
State Key Laboratory of Materials for Integrated Circuits, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China.
Selenium, as an important semiconductor material, exhibits significant potential for understanding lattice dynamics and thermoelectric applications through its thermal transport properties. Conventional empirical potentials are often unable to accurately describe the phonon transport properties of selenium crystals, which limits in-depth understanding of their thermal conduction mechanisms. To address this issue, this study developed a high-precision machine learning potential (MLP), with training datasets generated molecular dynamics simulations.
View Article and Find Full Text PDFNanomicro Lett
September 2025
State Key Laboratory of Bioinspired Interfacial Materials Science, School of Chemistry, Beihang University, Beijing, 100191, People's Republic of China.
Undesired ice accumulation on infrastructure and transportation systems leads to catastrophic events and significant economic losses. Although various anti-icing surfaces with photothermal effects can initially prevent icing, any thawy droplets remaining on the horizontal surface can quickly re-freezing once the light diminishes. To address these challenges, we have developed a self-draining slippery surface (SDSS) that enables the thawy droplets to self-remove on the horizontal surface, thereby facilitating real-time anti-icing with the aid of sunlight (100 mW cm).
View Article and Find Full Text PDFACS Omega
September 2025
Sinopec Key Laboratory of Research and Application of Medical and Hygienic Materials Sinopec (Beijing) Research Institute of Chemical Industry Co., Ltd., 14 Beisanhuan East Road, Chao Yang District, Beijing 100013, P. R. China.
With the rapid development of precision medicine and the continuous evolution of smart wearable devices, photothermal materials (PTMs) are experiencing a tremendous opportunity for growth. PTMs can efficiently convert light energy into heat to achieve localized thermal therapy for specific cells or tissues, offering advantages of minimal invasiveness, high selectivity, and precise targeting. Furthermore, PTMs can serve as molecular imaging probes and smart drug carriers, integrating multiple functions such as bioimaging and drug delivery to realize the visualization and controlled release of therapeutic processes.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
September 2025
School of Chemistry and Physics, Australian Research Council Research Hub in Zero-emission Power Generation for Carbon Neutrality, and Centre for Materials Science, Queensland University of Technology, Brisbane, QLD 4000, Australia.
Nanoporous structures play a critical role in a wide range of applications, including catalysis, thermoelectrics, energy storage, gas adsorption, and thermal insulation. However, their thermal instability remains a persistent challenge. Inspired by the extraordinary resilience of tardigrades, an "atomic armor" strategy is introduced to enhance the stability of nanoporous structures.
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