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We report about a new type of nonlinear photonic crystal fibers allowing broadband four-wave mixing and supercontinuum generation. The microstructured optical fiber has a structured core consisting of a rod of highly nonlinear glass material inserted in a silica tube. This particular structure enables four wave mixing processes with very large frequency detuning (>135 THz), which permitted the generation of a wide supercontinuum spectrum extending over 1650 nm after 2.15 m of propagation length. The comparison with results obtained from germanium-doped holey fibers confirms the important role of the rod material properties regarding nonlinear process and dispersion.
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http://dx.doi.org/10.1364/OE.17.015392 | DOI Listing |
ACS Omega
September 2025
Laboratório de Modelagem Molecular Aplicada e Simulação (LaMMAS), Universidade Estadual de Goiás, Anápolis, GO 75001-970, Brazil.
In this work, we report a theoretical investigation of the third-order nonlinear optical properties of the metronidazolium-picrate salt. The effects of the crystal environment are accounted for by the Iterative Charge Embedding approach, and the electronic calculations are carried out at the DFT (CAM-B3LYP/6-311++G-(d,p)) level. Furthermore, we use the results to parametrize a cavity Quantum Electrodynamics model for a quantum memory based on the Off-Resonant Cascaded Absorption protocol.
View Article and Find Full Text PDFRegulating the electronic structure by doping can promote photoluminescence emission of low-dimensional metal halides for developing white-light-emitting devices. Here, 0D metal halides RbBiCl have achieved a transition from nonluminescence to effective self-trapped excitons (STEs) emission after Sb ion doping at room temperature. The femtosecond transient absorption spectrum reveals the nonradiative recombination was suppressed, whose lifetimes change from 93.
View Article and Find Full Text PDFNano Lett
September 2025
Shaanxi Joint Lab of Graphene, State Key Laboratory of Photon-Technology in Western China Energy, International Collaborative Center on Photoelectric Technology and Nano Functional Materials, Institute of Photonics & Photon-Technology School of Physics Northwest University, Xi'an 710069, China.
The semiconductor-electrolyte interface with strong electrical tunability offers a platform for tuning nonlinear optical (NLO) processes and achieving giant optical nonlinearities. However, such a demonstration and fundamental mechanistic understanding of electrochemically tuned NLO properties have not been reported. Here, we developed an electrochemical Z-scan system to characterize the evolution of NLO responses in tellurium nanorod films under bias voltage.
View Article and Find Full Text PDFNat Nanotechnol
September 2025
Department of Physics and Astronomy, University of Pennsylvania, Philadelphia, PA, USA.
Topological photonics explores photonic systems that exhibit robustness against defects and disorder, enabled by protection from underlying topological phases. These phases are typically realized in linear optical systems and characterized by their intrinsic photonic band structures. Here we experimentally study Floquet Chern insulators in periodically driven nonlinear photonic crystals, where the topological phase is controlled by the polarization and the frequency of the driving field.
View Article and Find Full Text PDFCarbohydr Polym
November 2025
Molecular Imaging and Photonics, Department of Chemistry, KU Leuven, Campus Kulak Kortrijk, Etienne Sabbelaan 53, 8500 Kortrijk, Belgium. Electronic address:
Cellulose nanocrystals (CNCs) have emerged as promising candidates for chiroptical functional materials due to their ability to form cholesteric liquid crystals with tunable periodicity. The quality of the final cholesteric phase is influenced by the nucleation, growth and coalescence mechanism of the initial droplets, known as tactoids. Current research focuses on understanding the size and morphological transformations of these tactoids, to gain deeper insights into their dynamic behavior and, in turn, to better control the final properties of novel photonic materials.
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