ACS Photonics
August 2025
Triggered by advances in atomic-layer exfoliation and growth techniques, along with the identification of a wide range of extraordinary physical properties in self-standing films consisting of one or a few atomic layers, two-dimensional (2D) materials such as graphene, transition metal dichalcogenides (TMDs), and other van der Waals (vdW) crystals now constitute a broad research field expanding in multiple directions through the combination of layer stacking and twisting, nanofabrication, surface-science methods, and integration into nanostructured environments. Photonics encompasses a multidisciplinary subset of those directions, where 2D materials contribute remarkable nonlinearities, long-lived and ultraconfined polaritons, strong excitons, topological and chiral effects, susceptibility to external stimuli, accessibility, robustness, and a completely new range of photonic materials based on layer stacking, gating, and the formation of moiré patterns. These properties are being leveraged to develop applications in electro-optical modulation, light emission and detection, imaging and metasurfaces, integrated optics, sensing, and quantum physics across a broad spectral range extending from the far-infrared to the ultraviolet, as well as enabling hybridization with spin and momentum textures of electronic band structures and magnetic degrees of freedom.
View Article and Find Full Text PDFPhotonic integrated circuits (PICs) are transforming optical technology by miniaturizing complex photonic elements and systems onto single chips. However, scaling PICs to higher densities is constrained by optical crosstalk and device separation requirements, limiting both performance and size. Recent advancements in anisotropic metamaterials, particularly subwavelength gratings (SWGs), address these challenges by providing unprecedented control over evanescent fields and anisotropic perturbations in PICs.
View Article and Find Full Text PDFDigital detectors that "click" such as avalanche diodes and superconducting nanowire sensors are widely used in visible and near-infrared frequencies within the fields of quantum communications, imaging and metrology. On the other hand, the vast field of infrared bolometry has been dominated by analog detectors barring a few examples which require extremely challenging low temperature environments. Here, we propose and demonstrate a nanophotonic bolometer designed by engineering spintronic materials and dimensions to provide "clicks" from thermally activated transitions between two discrete magnetization states.
View Article and Find Full Text PDFRev Sci Instrum
February 2025
Tailoring optical and radiative properties has attracted significant attention recently due to its importance in advanced energy systems, nanophotonics, electro-optics, and nanomanufacturing. Metamaterials with micro- and nanostructures exhibit exotic radiative properties with tunability across the spectrum, direction, and polarization. Structures made from anisotropic or nanostructured materials have shown polarization-selective absorption bands in the mid-infrared.
View Article and Find Full Text PDFCarbon nanotube filaments with a twisted geometry emit spinning heat waves at high temperatures.
View Article and Find Full Text PDFDimensionality plays a crucial role in long-range dipole-dipole interactions (DDIs). We demonstrate that a resonant nanophotonic structure modifies the apparent dimensionality in an interacting ensemble of emitters, as revealed by population decay dynamics. Our measurements on a dense ensemble of interacting quantum emitters in a resonant nanophotonic structure with long-range DDIs reveal an effective dimensionality reduction to d[over ¯]=2.
View Article and Find Full Text PDFThe resolution of optical imaging is limited by diffraction as well as detector noise. However, thermal imaging exhibits an additional unique phenomenon of ghosting which results in blurry and low-texture images. Here, we provide a detailed view of thermal physics-driven texture and explain why it vanishes in thermal images capturing heat radiation.
View Article and Find Full Text PDFAnisotropic planar polaritons - hybrid electromagnetic modes mediated by phonons, plasmons, or excitons - in biaxial two-dimensional (2D) van der Waals crystals have attracted significant attention due to their fundamental physics and potential nanophotonic applications. In this Perspective, we review the properties of planar hyperbolic polaritons and the variety of methods that can be used to experimentally tune them. We argue that such natural, planar hyperbolic media should be fairly common in biaxial and uniaxial 2D and 1D van der Waals crystals, and identify the untapped opportunities they could enable for functional (i.
View Article and Find Full Text PDFACS Photonics
November 2023
The engineering of the spatial and temporal properties of both the electric permittivity and the refractive index of materials is at the core of photonics. When vanishing to zero, those two variables provide efficient knobs to control light-matter interactions. This Perspective aims at providing an overview of the state of the art and the challenges in emerging research areas where the use of near-zero refractive index and hyperbolic metamaterials is pivotal, in particular, light and thermal emission, nonlinear optics, sensing applications, and time-varying photonics.
View Article and Find Full Text PDFAll-optical switches control the amplitude, phase, and polarization of light using optical control pulses. They can operate at ultrafast timescales - essential for technology-driven applications like optical computing, and fundamental studies like time-reflection. Conventional all-optical switches have a fixed switching time, but this work demonstrates that the response-time can be controlled by selectively controlling the light-matter-interaction in so-called fast and slow materials.
View Article and Find Full Text PDFMachine perception uses advanced sensors to collect information about the surrounding scene for situational awareness. State-of-the-art machine perception using active sonar, radar and LiDAR to enhance camera vision faces difficulties when the number of intelligent agents scales up. Exploiting omnipresent heat signal could be a new frontier for scalable perception.
View Article and Find Full Text PDFSpinning thermal radiation is a unique phenomenon observed in condensed astronomical objects, including the Wolf-Rayet star EZ-CMa and the red degenerate star G99-47, due to the existence of strong magnetic fields. Here, by designing symmetry-broken metasurfaces, we demonstrate that spinning thermal radiation with a nonvanishing optical helicity can be realized even without applying a magnetic field. We design nonvanishing optical helicity by engineering a dispersionless band that emits omnidirectional spinning thermal radiation, where our design reaches 39% of the fundamental limit.
View Article and Find Full Text PDFEngineering symmetries in nanostructures and metasurfaces provides a new paradigm to control incoherent heat radiation for applications in energy conversion, thermal sources, infrared imaging, and radiative cooling.
View Article and Find Full Text PDFWe discover the quantum analog of the well-known classical maximum power transfer theorem. Our theoretical framework considers the continuous steady-state problem of coherent energy transfer through an N-node bosonic network coupled to an external dissipative load. We present an exact solution for optimal power transfer in the form of the maximum power transfer theorem known in the design of electrical circuits.
View Article and Find Full Text PDFA remarkable prediction of quantum field theory is that there are quantum electromagnetic fluctuations (virtual photons) everywhere, which leads to the intriguing Casimir effect. While the Casimir force between two objects has been studied extensively for several decades, the Casimir force between three objects has not been measured yet. Here, we report the experimental demonstration of an object under the Casimir force exerted by two other objects simultaneously.
View Article and Find Full Text PDFOpt Express
September 2022
We derive a unified quantum theory of coherent and incoherent energy transfer between two atoms (donor and acceptor) valid in arbitrary Markovian nanophotonic environments. Our theory predicts a fundamental bound = + for energy transfer efficiency arising from the spontaneous emission rates γ and γ of the donor and acceptor. We propose the control of the acceptor spontaneous emission rate as a new design principle for enhancing energy transfer efficiency.
View Article and Find Full Text PDFGeneration of a local magnetic field at the nanoscale is desirable for many applications such as spin-qubit-based quantum memories. However, this is a challenge due to the slow decay of static magnetic fields. Here, we demonstrate a photonic spin density (PSD)-induced effective static magnetic field for an ensemble of nitrogen-vacancy (NV) centers in bulk diamond.
View Article and Find Full Text PDFGermanium is typically used for solid-state electronics, fiber-optics, and infrared applications, due to its semiconducting behavior at optical and infrared wavelengths. In contrast, here we show that the germanium displays metallic nature and supports propagating surface plasmons in the deep ultraviolet (DUV) wavelengths, that is typically not possible to achieve with conventional plasmonic metals such as gold, silver, and aluminum. We measure the photonic band spectrum and distinguish the plasmonic excitation modes: bulk plasmons, surface plasmons, and Cherenkov radiation using a momentum-resolved electron energy loss spectroscopy.
View Article and Find Full Text PDFOne of the fundamental predictions of quantum mechanics is the occurrence of random fluctuations in a vacuum caused by the zero-point energy. Remarkably, quantum electromagnetic fluctuations can induce a measurable force between neutral objects, known as the Casimir effect, and it has been studied both theoretically and experimentally. The Casimir effect can dominate the interaction between microstructures at small separations and is essential for micro- and nanotechnologies.
View Article and Find Full Text PDFSpontaneous emission of quantum emitters can be enhanced by increasing the local density of optical states, whereas engineering dipole-dipole interactions requires modifying the two-point spectral density function. Here, we experimentally demonstrate long-range dipole-dipole interactions (DDIs) mediated by surface lattice resonances in a plasmonic nanoparticle lattice. Using angle-resolved spectral measurements and fluorescence lifetime studies, we show that unique nanophotonic modes mediate long-range DDI between donor and acceptor molecules.
View Article and Find Full Text PDFOver the past three decades, graphene has become the prototypical platform for discovering topological phases of matter. Both the Chern [Formula: see text] and quantum spin Hall [Formula: see text] insulators were first predicted in graphene, which led to a veritable explosion of research in topological materials. We introduce a new topological classification of two-dimensional matter - the optical N-phases [Formula: see text].
View Article and Find Full Text PDFSpin-momentum locking is a universal wave phenomenon promising for applications in electronics and photonics. In acoustics, Lord Rayleigh showed that surface acoustic waves exhibit a characteristic elliptical particle motion strikingly similar to spin-momentum locking. Although these waves have become one of the few phononic technologies of industrial relevance, the observation of their transverse spin remained an open challenge.
View Article and Find Full Text PDFImaging point sources with low angular separation near or below the Rayleigh criterion are important in astronomy, e.g., in the search for habitable exoplanets near stars.
View Article and Find Full Text PDFOver the past decade, topology has emerged as a major branch in broad areas of physics, from atomic lattices to condensed matter. In particular, topology has received significant attention in photonics because light waves can serve as a platform to investigate nontrivial bulk and edge physics with the aid of carefully engineered photonic crystals and metamaterials. Simultaneously, photonics provides enriched physics that arises from spin-1 vectorial electromagnetic fields.
View Article and Find Full Text PDFOpt Express
January 2020
Nearly all thermal radiation phenomena involving materials with linear response can be accurately described via semi-classical theories of light. Here, we go beyond these traditional paradigms to study a nonlinear system that, as we show, requires quantum theory of damping. Specifically, we analyze thermal radiation from a resonant system containing a χ nonlinear medium and supporting resonances at frequencies ω and ω ≈ 2ω, where both resonators are driven only by intrinsic thermal fluctuations.
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