Anaerobic digestion (AD) transforms organic waste into biogas, aligning with circular economy principles; however, its byproduct, digestate, poses waste management challenges due to variable composition and potential heavy metal contamination. This study proposes an innovative dual-purpose approach to convert waste digestate and air pollutants into energy. Solid digestate was pyrolyzed to produce high-performance biochar for toluene adsorption and subsequent use as solid recovered fuel (SRF), effectively valorizing waste materials.
View Article and Find Full Text PDFCarbon dioxide (CO) is a significant greenhouse gas that plays a pivotal role in driving global warming and climate change. Its primary sources stem from human activities, notably transportation, power generation, and industrial processes. Directly capturing CO emissions at their origins is widely recognized as a potent and efficient approach to reducing emissions.
View Article and Find Full Text PDFMercury (Hg)-contaminated farmlands have received wide attention because of the adverse risks posed to food security and human health. In addition, climate change altered the mobility of Hg in the soil, limiting soil productivity and nutrient bioavailability, hence elevating health risks. To adapt to these risks, pot experiments were employed to showcase the impacts of single-pyrolytic synthesized biochar with nitrogen and phosphorus impregnation (NPBC) on the nutrient accessibility, Hg immobilization, and human health risks, compared to pristine and control groups.
View Article and Find Full Text PDFAnthropogenic and industrial activities have released large amounts of mercury (Hg) into the hydrosphere. Hg ultimately deposits in sediments and could be re-released into the water environment, threatening the ecological system. Active capping is considered a suitable remediation method due to its relatively low cost and in-situ decontamination feasibility.
View Article and Find Full Text PDFPlatinum (Pt) and palladium (Pd) are commonly integrated into automotive catalytic converters to convert harmful emissions into relatively safer substances. Their scarcity has resulted in the rapid development of an industry focused on their recovery. Polyamide 6 (PA6), a microplastic pollutant, is a common industrial material.
View Article and Find Full Text PDFThe most common construction material used in Taiwan is concrete, potentially contaminated by geologic heavy metals (HMs). Younger children spend much time indoors, increasing HM exposure risks from household dust owing to their behaviors. We evaluated arsenic (As), cadmium (Cd), and lead (Pb) concentrations in fingernails among 280 preschoolers between 2017 and 2023.
View Article and Find Full Text PDFHealth risk assessments of exposure to mercury (Hg) from soils via ingestion and inhalation are indispensable for Taiwanese people living in the vicinity of Hg-contaminated sites. In this study, anthropogenic soils were collected from various polluted sources in Taiwan. In vitro oral and inhalation bioaccessible fractions of Hg were analyzed to avoid from overestimating the exposure risk.
View Article and Find Full Text PDFTrichloroethylene is carcinogenic and poorly degraded by microorganisms in the environment. Advanced Oxidation Technology is considered to be an effective treatment technology for TCE degradation. In this study, a double dielectric barrier discharge (DDBD) reactor was established to decompose TCE.
View Article and Find Full Text PDFBiofilters inoculated with activated sludge are widely used for odor control in WWTP. In this process, biofilm community evolution plays an important role in the function of reactor and is closely related to reactor performance. However, the trade-offs in biofilm community and bioreactor function during the operation are still unclear.
View Article and Find Full Text PDFDue to anthropogenic activities, heavy metals are discharged into the hydrosphere and deposit onto the sediment. Heavy metals remobilize through physical disturbance and change in environmental conditions, posing a risk to environments and human health. Among several remediation methods, active layer capping is considered to be more feasible due to its financial and technical advantages; however, its long-term effects remain unknown.
View Article and Find Full Text PDFHydrometallurgical processing of electronic waste produces copper (Cu)-containing wastewater. Recycling of Cu is thus crucial, as it reduces the Cu impact on the environment, and increases Cu sustainability in industry. Vacuum distillation provides excellent performance in both metals removal from aqueous solution, metal recovery, and metal impregnation to porous material.
View Article and Find Full Text PDFBackground: Controlling excess biomass accumulation and clogging is important for maintaining the performance of gas biofilters and reducing energy consumption. Interruption of bacterial communication (quorum quenching) can modulate gene expression and alter biofilm properties. However, whether the problem of excess biomass accumulation in gas biofilters can be addressed by interrupting bacterial communication remains unknown.
View Article and Find Full Text PDFThe elimination of volatile organic compounds (VOCs) emitted from the process of industry production is of great significance to improve the atmospheric environment. Herein the catalytic oxidation of the toluene and iso-hexane mixture, as the typical components from furniture paint industry, and the enhancement in the catalytic stability for toluene oxidation were investigated in detail. The formation rate of active oxygen species was very important for the development of the catalyst with high catalytic stability.
View Article and Find Full Text PDFMercury (Hg) is a well-known toxicant that can affect children's neurodevelopment. This study attempted to evaluate the internal dose of Hg in hair and fingernails and external Hg exposure from dietary consumption in 283 pairs of mothers and their children aged under 6 years in Taiwan. Mean Hg levels in hair and fingernail samples were 1.
View Article and Find Full Text PDFManganese oxide supported Pt single atoms (Pt/MnO) are prepared by the molten salt method. Catalytic oxidation of toluene and iso-hexane, typical emissions from furniture paints industry, is tested. Pt/MnO shows poor and high catalytic stability for toluene and iso-hexane oxidation, respectively.
View Article and Find Full Text PDFThis study focuses on estimating the probabilistic soil and dust ingestion rates for children under 3 years old by the Stochastic Human Exposure and Dose Simulation Soil and Dust (SHEDS-S/D) model developed by the U.S. Environmental Protection Agency.
View Article and Find Full Text PDFWet flue gas desulfurization (WFGD) simultaneously removes Hg and SO from coal-fired power plant flue gas streams. Hg re-emission occurs when the dissolved Hg(II) is converted to a volatile form (i.e.
View Article and Find Full Text PDFDue to public health threats resulting from mercury (Hg) and its distribution in the food chain, global restrictions have been placed on Hg use and emissions. Biochar is a porous, carbonaceous adsorbent typically derived from waste biomass or organic matter, making it an eco-friendly material for aqueous mercury (Hg(II)) control. Functionalization of biochar can improve performance in pollution control applications.
View Article and Find Full Text PDFLead (Pb) exposure increases the risks of neurodevelopmental disorders in children. Child-specific activities and land use scenarios may lead to elevated opportunities for Pb exposure through the soil. Therefore, we investigated hair and fingernail Pb concentrations among young children in northern Taiwan, in relation to soil Pb pollution and land use characteristics.
View Article and Find Full Text PDFSci Total Environ
July 2021
Odor emissions from intensive livestock farms have attracted increased attention due to their adverse impacts on the environment and human health. Nevertheless, a systematic summary regarding the characteristics, sampling detection, and control technology for odor emissions from livestock farms is currently lacking. This paper compares the development of odor standards in different countries and summarizes the odor emission characteristics of livestock farms.
View Article and Find Full Text PDFIn this study, the mercury (Hg) emission, speciation, and mass distribution of four coal-fired power plants (CFPPs) located at central, southern, and northern Taiwan with various types of air pollution control devices were investigated. Gaseous Hg in the coal-combustion flue gas was sampled by using the Ontario Hydro method, and the solid and liquid samples were collected for understanding the Hg mass balance. The experimental results showed that the total Hg concentrations in flue gases at the inlets of selective catalytic reduction (SCR) varied from 2.
View Article and Find Full Text PDFA novel electrothermal swing (ETS) system with gold-electrodeposited activated carbon fiber cloth (GE-ACFC) was developed to adsorb and sustainably recover low-concentration Hg. GE-ACFC with an Au growth time of 1200 s displayed the largest Hg adsorption capacity and >90% removal efficiency. The Hg adsorption of GE-ACFC was dominated by physisorption via Au amalgamation.
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