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http://dx.doi.org/10.1016/j.scib.2025.08.027 | DOI Listing |
Nanoscale
September 2025
School of Materials Science and Engineering, Beihang University, Beijing 100191, China.
The challenge of photocatalytic hydrogen production has motivated a targeted search for MXenes as a promising class of materials for this transformation because of their high mobility and high light absorption. High-throughput screening has been widely used to discover new materials, but the relatively high cost limits the chemical space for searching MXenes. We developed a deep-learning-enabled high-throughput screening approach that identified 14 stable candidates with suitable band alignment for water splitting from 23 857 MXenes.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2025
Department of Organic and Nano Engineering, and Human-Tech Convergence Program, Hanyang University, 222 Wangsimni-ro, Seongdong-gu, Seoul 04763, Republic of Korea.
Photomultiplication-type organic photodetectors (PM-type OPDs) have recently attracted attention. However, the development of polymer donors specifically tailored for this architecture has rarely been reported. In this study, we synthesized benzobisoxazole-based polymer donors incorporating alkylated π-spacers that simultaneously enhance photocurrent density () and suppress dark current density (), leading to high responsivity () and specific detectivity (*).
View Article and Find Full Text PDFAdv Mater
September 2025
Center of Electron Microscopy, State Key Laboratory of Silicon and Advanced Semiconductor Materials, School of Materials Science and Engineering, Zhejiang Key Laboratory of Low-Carbon Synthesis of Value-Added Chemicals, Zhejiang University, Hangzhou, 310027, China.
Electrocatalysis, a pivotal field at the intersection of physical chemistry and materials science, plays a crucial role in advancing energy conversion and storage technologies through rational catalyst design. However, understanding reaction mechanisms at the atomic level remains a great challenge due to the intricate interplay between catalysts, reactants, and complex environments (e.g.
View Article and Find Full Text PDFSmall
September 2025
Institute of Chemistry, Academia Sinica, Taipei, 115201, Taiwan.
Achieving high capacitance while maintaining rapid charge transport and structural stability remains a major challenge in the design of battery-type supercapacitor electrodes. Herein, a molecularly engineered strategy is presented for constructing hierarchical hybrid electrodes by integrating petal-like NiCu-LDH nanosheets onto 3D HBC-x (x = H, F, OMe)-functionalized CNT paper via a one-step hydrothermal process. The incorporation of HBC effectively mitigates CNT agglomeration and constructs an interconnected conductive framework that enhances charge transport, shortens ion diffusion paths, and reduces internal resistance.
View Article and Find Full Text PDFAdv Mater
September 2025
School of Physical Science and Technology, College of Energy, School of Optoelectronic Science and Engineering, Soochow University, Suzhou, 215000, P. R. China.
Polymer additives exhibit unique advantages in suppressing lead leaching from perovskite solar cells (PSCs). However, polymers tend to excessively aggregate in the perovskite film, which hinders comprehensive encapsulation and disrupts charge transport efficiency, degrading lead leakage inhibition and device performance. Herein, a polymer dynamic soft encapsulation strategy driven by molecular extrusion is introduced to mitigate lead leakage in PSCs, achieved through the incorporation of poly(propylene adipate) (PPA) as a multifunctional additive in the perovskite formulation.
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