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We present a novel dual-functional surface design that strategically integrates superhydrophobic and lubricant-infused surface technologies to achieve switchable liquid repellency with significantly enhanced durability and self-healing capabilities. By precisely controlling the amount of silicone oil infused─quantified as surface loading─into laser-induced graphene structures on polyimide substrates, we demonstrate a controlled transition between superhydrophobic and lubricant-infused states. This hybrid approach effectively addresses the critical challenges of both technologies: the mechanical vulnerability of superhydrophobic surfaces and lubricant depletion issues in lubricant-infused surfaces. Our systematic investigation reveals an optimal silicone oil loading that maintains excellent water repellency even after substantial surface damage, evidenced by high contact angles and low sliding angles across damaged regions of up to 2 mm in width. The self-healing mechanism provided by the strategic lubricant layer preserves liquid-repellent properties after physical damage, significantly outperforming conventional superhydrophobic surfaces in durability tests. Experimental results using candle-soot-treated surfaces further confirm the superior damage resistance of our hybrid design. This work provides new insights into liquid-repellent surface engineering with potential applications in self-cleaning coatings, anti-icing surfaces, oil-water separation, and microfluidic devices that require sustained performance in harsh environments.
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http://dx.doi.org/10.1021/acs.langmuir.5c02261 | DOI Listing |
Cell Biol Int
July 2025
Department of Biophysics, Friedrich-Alexander-Universität Erlangen-Nürnberg, Erlangen, Germany.
Traditional treatment of biofouling with toxic paints or antibiotics has significant limitations and challenges, including negative impacts on surrounding ecosystems and the emergence of resistant microbial strains. Antibiotics often prove ineffective in penetrating the dense and protective structure of biofilms, rendering traditional antimicrobial approaches less effective and leading to chronic infections. Toxic paints, while initially effective in reducing microbial colonization, contribute to long-term environmental contamination and harm non-target organisms.
View Article and Find Full Text PDFLangmuir
September 2025
Institute of Applied Mechanics, National Taiwan University, No.1, Sec. 4, Roosevelt Rd., Da'an Dist., Taipei 106, Taiwan (R.O.C.).
We present a novel dual-functional surface design that strategically integrates superhydrophobic and lubricant-infused surface technologies to achieve switchable liquid repellency with significantly enhanced durability and self-healing capabilities. By precisely controlling the amount of silicone oil infused─quantified as surface loading─into laser-induced graphene structures on polyimide substrates, we demonstrate a controlled transition between superhydrophobic and lubricant-infused states. This hybrid approach effectively addresses the critical challenges of both technologies: the mechanical vulnerability of superhydrophobic surfaces and lubricant depletion issues in lubricant-infused surfaces.
View Article and Find Full Text PDFACS Appl Mater Interfaces
May 2025
Energy Transport Lab, Department of Mechanical Engineering, University of Michigan, Ann Arbor, Michigan 48109, United States.
Understanding droplet-surface interactions has broad implications in microfluidics and lab-on-a-chip devices. In contrast to droplets on conventional textured air-filled superhydrophobic surfaces, water droplets on state-of-the-art lubricant-infused surfaces are accompanied by an axisymmetric annular wetting ridge, the source and nature of which are not clearly established to date. Generally, the imbalance of interfacial forces at the contact line is believed to play a pivotal role in accumulating the lubricant oil near the droplet base to form the axisymmetric wetting ridge.
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July 2024
School of Mechanical and Aerospace Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore.
The greater geometrical design freedom offered by additive manufacturing (AM) as compared to the conventional manufacturing method has attracted increasing interest in AM to develop innovative and complex designs for enhanced performance. However, the difference in material composition and surface properties from conventional alloys has made surface micro-/nanostructuring of AM metals challenging. Frost accretion is a safety hazard in numerous engineering applications.
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March 2024
College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin 150001, China.
The superhydrophobic surface and slippery liquid-infused porous surface (SLIPS)/lubricant-infused surface (LIS) have attracted increasing attention owing to their multifunctionality. However, their practical applications face several problems such as complex and inefficient preparation technology, loss of lubricant, and fragile microstructures. Therefore, new strategies for preparing microstructures must be developed for constructing superhydrophobic and lubricant-infused coatings.
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