98%
921
2 minutes
20
Generation of broadband terahertz (THz) pulses with variable polarization and carrier-envelope phase can enable the tailoring of THz beam wavefronts for advanced applications in THz imaging and spectroscopy and for strong THz field optics. While metasurfaces composed of deeply subwavelength THz emitters have recently been demonstrated to define the polarization and spatial profile of the generated THz fields, precise phase control or synthesis of THz pulse waveforms remains a challenging problem. Here, we propose and demonstrate metasurfaces composed of indium arsenide (InAs) nanoscale ribbon arrays capable of generating THz pulses with variable carrier-envelope phase. We show that different THz generation mechanisms, each contributing distinct phases, can be activated in the ribbons, enabling carrier-envelope phase control spanning a range of π over a wide band of frequencies (∼1-3 THz). This is achieved solely through the ribbon array geometry using linearly polarized optical excitation of the ribbons. The arrays enable precise control of the THz phase and amplitude, opening the door to advanced structured THz wavefront synthesis using ultrathin dielectric metasurfaces.
Download full-text PDF |
Source |
---|---|
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC12372169 | PMC |
http://dx.doi.org/10.1021/acsphotonics.5c00941 | DOI Listing |
ACS Photonics
August 2025
Electronic and Electrical Engineering, University College London, Torrington Place, London WC1E 7JE, U.K.
Generation of broadband terahertz (THz) pulses with variable polarization and carrier-envelope phase can enable the tailoring of THz beam wavefronts for advanced applications in THz imaging and spectroscopy and for strong THz field optics. While metasurfaces composed of deeply subwavelength THz emitters have recently been demonstrated to define the polarization and spatial profile of the generated THz fields, precise phase control or synthesis of THz pulse waveforms remains a challenging problem. Here, we propose and demonstrate metasurfaces composed of indium arsenide (InAs) nanoscale ribbon arrays capable of generating THz pulses with variable carrier-envelope phase.
View Article and Find Full Text PDFApproaches for efficient pulse compression can enable dramatic increases in the available peak power, as well as enable the generation of isolated attosecond X-ray pulses. Achieving high compression ratios for longer wavelength drivers has, however, been challenging. We present the compression of few-cycle 2.
View Article and Find Full Text PDFOpt Express
February 2025
Dual-comb spectroscopy (DCS) has emerged as an indispensable optical technique for probing broadband optical spectra of molecular species with high resolution. To better understand the impact of phase noise in free-running DCS implementations, we investigate the effects of timing jitter and carrier-envelope phase noise on the shape of Lorentzian absorption lines extracted from single-shot interferograms. An analysis of linewidth broadening and fluctuations of the center frequency allows us to quantify the amount of optical frequency comb noise that significantly distorts absorption features.
View Article and Find Full Text PDFThe carrier-envelope phase () of few-cycle light pulses is of crucial importance for strong-field light-matter interaction on subcycle time scales. Standard -2 interferometry rapidly records beat notes defined by the carrier-envelope offset frequency (), but measuring at a high bandwidth is more involved. Here, we introduce -2 polarization interferometry, which unambiguously measures over a range of 2π at the detection speed of the implemented photodiodes.
View Article and Find Full Text PDFUsing the solution of the time-dependent Schrödinger equation beyond the Born-Oppenheimer approximation, we investigate high-order harmonic generation of the hydrogen molecular ion (H2+) in a few-cycle chirped laser pulse. Our results demonstrate that a double-plateau structure in the high-order harmonic spectra shows up for H2+ subjected to a few-cycle chirped laser field when the chirp parameter changes from negative to positive. Theoretical analysis indicates that the dependence of the double-plateau structure on the chirp of the laser pulse is primarily attributed to the influence of quantum diffusion effects.
View Article and Find Full Text PDF