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Magnetic skyrmionic structures, including magnetic skyrmions and antiskyrmions, are characterized by swirling spin textures with non-trivial topologies. They are featured with specific topological charges, Q, which are of crucial importance in determining their topological properties. Owing to the invariance of the chiral nature, it is generally believed that Q is conserved in a given magnetic skyrmionic structure and is hard to alter. Here, we experimentally realize the control of Q of magnetic skyrmionic structures at room temperature in a Dzyaloshinskii-Moriya interaction (DMI) platform with spatially alternating signs. Depending on how many times it crosses the interfaces between DMI regions with opposite signs, the magnetic skyrmionic structures possess different Q. Modifying the DMI energy landscape through chemisorbed oxygen, a magnetic topological transition is realized. This creation and manipulation of magnetic skyrmionic structures with controllable Q, in particular the DMI-stabilized thin-film antiskyrmions and high-Q skyrmionic structures, enables a new degree of freedom to control their dynamics via a novel DMI confinement effect. Our findings open up an unexplored avenue on various topological magnetic skyrmionic structures and their potential applications.
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http://dx.doi.org/10.1038/s41467-025-58529-4 | DOI Listing |
ACS Nano
September 2025
Ultrafast Electron Microscopy Laboratory, The MOE Key Laboratory of Weak-Light Nonlinear Photonics, School of Physics, Nankai University, Tianjin 300071, China.
Superlattices (SLs) based on two-dimensional (2D) van der Waals (vdW) materials, abbreviated as 2D-SLs, have garnered significant attention due to their customizable properties. 2D-SLs can be engineered by mechanical stacking or chemical intercalation to achieve diverse forms of symmetry breaking, resulting in exotic phenomena like the quantum anomalous Hall effect and topological magnetism. Hitherto, broken symmetries in 2D-SLs have been widely produced within lateral planes or three dimensions.
View Article and Find Full Text PDFNano Lett
September 2025
Department of Physics and Astronomy and California NanoSystems Institute, University of California, Los Angeles, California 90095, United States.
Moiré superlattices introduce new length and energy scales, enabling discoveries, such as unconventional superconductivity, in 2D systems. This concept has recently been extended to bulk materials with multiple- spin textures, opening exciting opportunities for spin moiré physics. A notable example is EuAgSb, where a spin moiré superlattice (SMS), manifested as a double- spin modulation, induces a superzone gap opening.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
Department of Electrical and Electronics Engineering, Koç University, Sariyer, Istanbul 34450, Turkey.
Skyrmion-based devices promise energy-efficient spintronic functionalities, but polycrystalline magnetic films can degrade performance by inducing skyrmion pinning. Here, we use micromagnetic modeling to quantify the impact of polycrystallinity-induced variability in key material parameters such as saturation magnetization, Dzyaloshinskii-Moriya interaction, and uniaxial anisotropy on skyrmion stability, dynamics, and hysteresis loops in Co/Pt films and device geometries. We demonstrate that variations exceeding 5% in these parameters across grains significantly increase the likelihood of pinning, with the effects depending on both grain size and distribution.
View Article and Find Full Text PDFSci Rep
August 2025
Crystal Growth Facility, École Polytechnique Fédérale de Lausanne, SB, IPHYS, 1015, Lausanne, Switzerland.
The formation and characteristics of magnetic skyrmions are strongly governed by the symmetry of the underlying crystal structure. In this study, we report the discovery of a new trigonal polymorph of CuOSeO, observed exclusively in nanoparticles. Electron diffraction and density functional theory calculations confirm its R3m space group, sharing C symmetry with Néel-type skyrmion hosts.
View Article and Find Full Text PDFSmall
August 2025
Institute of Advanced Magnetic Materials, College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou, 310012, China.
Kagomé lattice magnets have recently garnered significant interest due to the pronounced transverse transport characteristics, particularly in thermoelectric and spintronic applications, stemming from the interplay between topology and magnetism. Here, a comprehensive investigation of the magnetic, electrical, and thermoelectric transport properties, as well as the complex spin configurations, is conducted in a polycrystalline Kagomé ferromagnet GdCo. Strikingly, a giant anomalous Hall conductivity ≈2125 S cm is obtained at T = 10 K, which is primarily governed by the extrinsic skew-scattering mechanism.
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