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Article Abstract

The fractional quantum anomalous Hall (FQAH) effect was recently discovered in twisted MoTe (tMoTe) bilayers. Experiments so far have revealed Chern insulators from hole doping at ν = -1, -2/3, -3/5 and -4/7 (per moiré unit cell). In parallel, theories predict that, between v = -1 and -3, there exist exotic quantum phases, such as the coveted fractional topological insulators, fractional quantum spin Hall (FQSH) states and non-Abelian fractional states. Here we use transient optical spectroscopy on tMoTe to reveal nearly 20 hidden states at fractional fillings that are absent in static optical sensing or transport measurements. A pump pulse selectively excites charge across the correlated or pseudogaps, leading to the disordering (melting) of correlated states. A probe pulse detects the subsequent melting and recovery dynamics by means of exciton and trion sensing. Besides the known states, we observe further fractional fillings between ν = 0 and -1 and a large number of states on the electron doping side (ν > 0). Most importantly, we observe new states at fractional fillings of the Chern bands at ν = -4/3, -3/2, -5/3, -7/3, -5/2 and -8/3. These states are potential candidates for the predicted exotic topological phases. Moreover, we show that melting of correlated states occurs on two distinct timescales, 2-4 ps and 180-270 ps, attributed to electronic and phonon mechanisms, respectively. We discuss the differing dynamics of the electron-doped and hole-doped states from the distinct moiré conduction and valence bands.

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http://dx.doi.org/10.1038/s41586-025-08954-8DOI Listing

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