Deep-learning approach for developing bilayered electromagnetic interference shielding composite aerogels based on multimodal data fusion neural networks.

A non-experimental approach to developing high-performance EMI shielding materials is urgently needed to reduce costs and manpower. In this investigation, a multimodal data fusion neural network model is proposed to predict the EMI shielding performances of silver-modified four-pronged zinc oxide/waterborne polyurethane/barium ferrite (Ag@F-ZnO/WPU/BF) aerogels. First, 16 Ag@F-ZnO/WPU/BF samples with varying Ag@F-ZnO and BF contents were successfully prepared using the pre-casting and directional freezing techniques. The experimental results demonstrate that these aerogels perform well in terms of averaged EMI shielding effectiveness (SE) up to 78.6 dB and absorption coefficient as high as 0.96. On the basis of composite ingredients and microstructural images, the established multimodal neural network model can effectively predict the EMI shielding performances of Ag@F-ZnO/WPU/BF aerogels. Notably, the multimodal model of fully connected neural network (FCNN) and residual neural network (ResNet) utilizing GatedFusion method yields the best root mean squared error (RMSE) and mean absolute error (MAE) values of 0.7626 and 0.4918, respectively, and correlation coefficient (R) of 0.9885. In addition, this multimodal model successfully predicts the EMI performances of four new aerogels with an average error of less than 5 %, demonstrating its strong generalization capability. The accuracy and efficiency of material property prediction based on multimodal neural network model are largely improved by integrating multiple data sources, offering new possibility for reducing experimental burdens, accelerating the development of new materials, and gaining a deeper understanding of material mechanisms.