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Borophene, owing to the high mobility and long spin coherent length of its carriers, presents significant opportunities in ultrafast spintronics. In this research, we investigate the spin-dependent conductance of a Datta-Das field-effect transistor (FET) based on an armchair β-borophene nanoribbon (BNR) using the tight-binding (TB) Hamiltonian in combination with the non-equilibrium Green's function (NEGF) method. The spin FET electrodes are magnetized by ferromagnetic (FM) insulators arranged in both parallel and anti-parallel configurations. This device acts as a controllable spin filter in the presence of Rashba spin-orbit coupling (SOC) for both configurations and its spin current is well modulated by a gate voltage and the strength of the Rashba SOC. For anti-parallel configurations, an energy gap emerges within a certain range of incoming electron energy which can disappear for electrons with flipped spin under the Rashba SOC. Furthermore, our findings indicate that the electron-electron (e-e) interaction helps the spin precession of electrons injected into the spin FET channel, thereby strengthening the Rashba SOC effect. Notably, a gate voltage can adjust the current-voltage (-) characteristics of this device. Finally, our calculations demonstrate that under the same conditions, the current magnitude and / ratio of borophene spin FETs are several times higher than those of graphene and silicene spin FETs.
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http://dx.doi.org/10.1039/d4cp00239c | DOI Listing |
Nano Lett
September 2025
Key Laboratory of Micro & Nano Photonic Structures, Department of Optical Science and Engineering, College of Future Information Technology, Fudan University, Shanghai 200433, China.
The separation and propagation of spin are vital to understanding spin-orbit coupling (SOC) in quantum systems. Exciton-polaritons, hybrid light-matter quasiparticles, offer a promising platform for investigating SOC in quantum fluids. By utilization of the optical anisotropy of materials, Rashba-Dresselhaus SOC (RDSOC) can be generated, enabling robust polariton spin transport.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
Department of Nanotechnology for Sustainable Energy, School of Science and Technology, Kwansei Gakuin University, 1 Gakuen-Uegahara, Sanda 669-1330, Japan.
Monolayer Janus transition-metal dichalcogenides possess Ising- and Rashba-type spin-orbit-couplings (SOC), leading to intriguing spin splitting effects at K and K', and around Γ points across the wide energy range. Using first-principles calculations, we unveil these SOC characteristics in metallic Janus NbSSe and demonstrate its potential for optically controlled spin current generation. On the basis of the symmetry of the system, we show that different linear polarized light can selectively drive spin currents of distinct spin components.
View Article and Find Full Text PDFACS Nano
September 2025
Department of Chemical and Biological Engineering, University of Colorado, Boulder, Colorado 80303, United States.
Tuning the exciton fine structure of lead halide perovskites to brighten the dark excitonic ground state is crucial for enhancing their optoelectronic performance. While Rashba splitting is linked to dark-to-light exciton flipping, the specific nature of this phenomenon remains unclear. Here, we systematically studied 18 CsPbBr structures, representing 2D systems of CsPbBr with varying degrees of distortion, using density functional theory (DFT) and the Model-Bethe-Salpeter Equation (m-BSE).
View Article and Find Full Text PDFJ Chem Phys
August 2025
School of Physics and Physical Engineering, Qufu Normal University, Qufu 273165, China.
Three-dimensional lead halide perovskites (3D LHPs) exhibit giant Rashba spin-orbit coupling (SOC) due to their inherent lattice asymmetry and heavy-metal composition; yet, the impact of Rashba SOC on the luminescence dynamic of 3D LHPs remains debated. Here, we utilize the magneto-photoluminescence (Magneto-PL) effects as an effective tool to reveal the underlying spin-related opto-physical process in 3D LHPs. We find that the magneto-PL effects of 3D LHPs CH3NH3Pb(Br/I/IxCl1-x)3 thin films are negative and tunable at room temperature, indicating the remarkable suppression of their PL emission intensity by magnetic fields.
View Article and Find Full Text PDFJ Am Chem Soc
August 2025
Department of Chemistry, University of Utah, Salt Lake City, Utah 84112, United States.
Chiral hybrid organic-inorganic semiconductors (CHOIS), which integrate chiral organic cations by hydrogen-bonding interactions with anionic metal halide subunits, have recently emerged as cutting-edge materials with the potential to revolutionize energy-efficient information processing, particularly in the realms of spintronics. By harnessing the inherent chirality of organic cations, CHOIS can effectively manipulate spin dynamics, a crucial factor for enhancing the device performance in next-generation electronics. However, the challenge lies in the limited understanding of structure-property relationships, which hinders the ability to control and fine-tune the chirality within these materials.
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