Universal Evolution of Fickian Non-Gaussian Diffusion in Two- and Three-Dimensional Glass-Forming Liquids.

Int J Mol Sci

Department of Chemical, Materials and Production Engineering, University of Naples Federico II, P.le Tecchio 80, 80125 Napoli, Italy.

Published: April 2023


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Article Abstract

Recent works show that glass-forming liquids display Fickian non-Gaussian Diffusion, with non-Gaussian displacement distributions persisting even at very long times, when linearity in the mean square displacement (Fickianity) has already been attained. Such non-Gaussian deviations temporarily exhibit distinctive exponential tails, with a decay length λ growing in time as a power-law. We herein carefully examine data from four different glass-forming systems with isotropic interactions, both in two and three dimensions, namely, three numerical models of molecular liquids and one experimentally investigated colloidal suspension. Drawing on the identification of a proper time range for reliable exponential fits, we find that a scaling law λ(t)∝tα, with α≃1/3, holds for all considered systems, independently from dimensionality. We further show that, for each system, data at different temperatures/concentration can be collapsed onto a master-curve, identifying a characteristic time for the disappearance of exponential tails and the recovery of Gaussianity. We find that such characteristic time is always related through a power-law to the onset time of Fickianity. The present findings suggest that FnGD in glass-formers may be characterized by a "universal" evolution of the distribution tails, independent from system dimensionality, at least for liquids with isotropic potential.

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http://www.ncbi.nlm.nih.gov/pmc/articles/PMC10177888PMC
http://dx.doi.org/10.3390/ijms24097871DOI Listing

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