Cosmogenic Be: Particle size distribution and chemical composition of Be-carrying aerosols in the atmosphere in Japan.

J Environ Radioact

Central Institute of Radioisotope Science and Safety Management, Kyushu University (Professor Emeritus), 744 Motooka, Fukuoka, 819-0395, Japan.

Published: October 2021


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Article Abstract

The particle size distributions of airborne aerosols with Be were measured using cascade impactors at Dazaifu, a city in western Japan, in 2018 to observe their seasonal variation. Beryllium-7 was found to be adsorbed to aerosols with a particle size of less than 2.1 μm; in general, particles sized 0.43-0.65 μm had the highest Be activity concentrations. The activity median aerodynamic diameter (AMAD) of Be fluctuated less over the year within the range of 0.40-0.52 μm, which is the size range of particles that can reach human alveoli, and had an annual mean of 0.43 ± 0.034 μm. The activity concentrations of Be were significantly lower in summer, which affected Be activity concentration for each particle size fraction. The particle size distribution of Be-carrying aerosols was also affected by that of the aerosol particles in the atmosphere. Finally, findings suggest that Be was mainly adsorbed to sulfate aerosols (particularly ammonium sulfate aerosols).

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http://dx.doi.org/10.1016/j.jenvrad.2021.106690DOI Listing

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