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Solar steam generation is considered as an efficient way for addressing water shortage issues seawater desalination and wastewater purification. In a solar evaporator, an absorber would convert optical energy to heat for evaporating nearby water. In this process, many low-boiling-point contaminants can also be evaporated along with water steam, which compromises the effectiveness of purification. There is, so far, no study on the removal of such low-boiling-point contaminants such as organic pesticides in wastewater. To address this problem, we demonstrate a versatile carbon hybrid aerogel (CHA) as a solar powered water purification platform. With an elaborate absorber design, the maximum solar evaporation rate of 2.1 kg m h is achieved under 1 sun illumination. More importantly, CHA can effectively suppress the evaporation of low-boiling-point contaminants including common pesticides and mercury ion its strong adsorption and retention effect. Synergetic steaming and the adsorption of CHA will inspire more paradigms of solar steam generation technologies for applications relevant to detoxification and water remediation.
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http://dx.doi.org/10.1021/acsami.1c06000 | DOI Listing |
Nano Lett
June 2023
Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials (Ministry of Education), School of Materials Science and Engineering, Shandong University, Jinan 250061, People's Republic of China.
MXenes are emerging 2D materials that have gained great attention because of their unique physical-chemical properties. However, the wide application of MXenes is prohibited by their high cost and environmentally harmful synthesis process. Here a fluoride- and acid-free physical vacuum distillation strategy is proposed to directly synthesize a series of MXenes.
View Article and Find Full Text PDFSe Pu
January 2023
College of Chemistry and Chemical Engineer, Xinjiang Normal University, Urumqi 830054, China.
ACS Appl Mater Interfaces
July 2021
Center of Super-Diamond and Advanced Films (COSDAF) & Department of Chemistry, City University of Hong Kong, 83 Tat Chee Avenue, Kowloon, Hong Kong SAR, P. R. China.
Solar steam generation is considered as an efficient way for addressing water shortage issues seawater desalination and wastewater purification. In a solar evaporator, an absorber would convert optical energy to heat for evaporating nearby water. In this process, many low-boiling-point contaminants can also be evaporated along with water steam, which compromises the effectiveness of purification.
View Article and Find Full Text PDFFood Chem
October 2021
Pesticide Safety Evaluation Research Center, Institute for Agro-food Standards and Testing Technology, Shanghai Academy of Agricultural Sciences, Shanghai 2011106, China. Electronic address:
An innovative method was established for the determination of 1-methylcyclopropene (1-MCP) in vegetables and fruits. Due to its small molecular weight and low boiling point, it was difficult to obtain quantitative analysis for 1-MCP, especially at the residual level. In this work, based on its iodine derivatives, 1-MCP was derived to 1,2-diiodo-1-methylcyclopropane, which was much easier for trace and accurate chromatographic analysis.
View Article and Find Full Text PDFACS Omega
November 2020
College of Biological, Chemical Sciences and Engineering, Jiaxing University, 118 Jiahang Road, Jiaxing 314001, China.
Two types of SO /ZrO solid acid catalysts with various calcination times were prepared via incipient wetness impregnation of (NH)SO to hydrothermally synthesized ZrO and subsequently employed to catalyze the esterification of palmitic acid with methanol. The resulting catalysts were characterized by X-ray diffraction (XRD), Fourier transform infrared (FTIR) spectroscopy, and temperature-programmed oxidation (TPO) to elucidate their physicochemical properties, morphology, and deactivation mechanism. A calcination procedure is required to transform the amorphous ZrO into the crystal form.
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