Category Ranking
98%
Total Visits
921
Avg Visit Duration
2 minutes
Citations
20
Article Abstract
To mimic and use the functions of the ion transport system that are central to biological processes, bioinspired ion-selective membranes are developed and show great potential in a variety of fields. However, the practical applications of them are now limited due to low pore density, low conductivity, or scale-up difficulty. Herein, we demonstrate a 2-hydroxyethyl methacrylate phosphate (HEMAP) hydrogel membrane with 3D interconnected nanopores and space charged through simple photopolymerization. The HEMAP hydrogel membrane exhibits high conductance and outstanding ion selectivity, and the membrane-based osmotic power generator shows the excellent output power density up to 5.38 W/m. Both experimentally and theoretically, the 3D interconnected structure is revealed to play a key role in enhancing charge-governed ion transport and energy conversion. This work highlights the advantages of 3D interconnected nanopores in ion diffusion and shows the potential of our designed hydrogel membrane in osmotic energy conversion, water desalination, and sensors.
Download full-text PDF |
Source |
|---|---|
| http://dx.doi.org/10.1021/acs.nanolett.0c01087 | DOI Listing |
Publication Analysis
Top Keywords
Similar Publications
Combating the post-antibiotic era crisis: antimicrobial peptide/peptidomimetic-integrated combination therapies and delivery systems.
J Mater Chem B
September 2025
State Key Laboratory of Bioactive Molecules and Druggability Assessment, Guangdong Basic Research Center of Excellence for Natural Bioactive Molecules and Discovery of Innovative Drugs, College of Pharmacy, Jinan University, Guangzhou 511436, China.
Globally, new antibiotic development lags behind the rapid evolution of antibiotic-resistant bacteria. Given the extensive research and development cycles, high costs, and risks associated with new pharmaceuticals, exploring alternatives to conventional antibiotics and enhancing their efficacy and safety is a promising strategy for addressing challenges in the post-antibiotic era. Previous studies have shown that antimicrobial peptides/peptidomimetics (AMPs) primarily use a membrane-disruption mechanism distinct from conventional antibiotics to exert bactericidal effects.
View Article and Find Full Text PDFProto-SLIPS: Slippery Liquid-Infused Surfaces that Release Highly Water-Soluble Agents.
ACS Appl Mater Interfaces
September 2025
Department of Chemistry, University of Wisconsin-Madison, 1101 University Ave., Madison, Wisconsin 53706, United States.
Slippery liquid-infused porous surfaces (or "SLIPS") can prevent bacterial surface fouling, but they do not inherently possess the means to kill bacteria or reduce cell loads in surrounding media. Past reports show that the infused liquids in these materials can be leveraged to load and release antimicrobial agents, but these approaches are generally limited to the use of hydrophobic agents that are soluble in the infused oily phases. Here, we report the design of so-called "proto-SLIPS" that address this limitation and permit the release of highly water-soluble (or oil-insoluble) agents.
View Article and Find Full Text PDFTheoretical simulation-guided design and fabrication of molecularly imprinted hydrogels for selective osteopontin separation.
Food Res Int
November 2025
State Key Laboratory of Marine Food Processing & Safety Control, College of Food Science and Engineering, Ocean University of China, Qingdao, 266003, China. Electronic address:
Osteopontin (OPN), a multifunctional milk protein essential for bioactive functions, remains challenging to isolate efficiently due to the limited specificity of conventional methods. We developed hydrogel-based molecularly imprinted membranes (MIMs) for selective OPN recognition. Dimethylaminopropyl methacrylamide (DMAPMA) and N-isopropylacrylamide (NIPAM) were selected as functional monomers based on molecular docking and molecular dynamics (MD) simulations, ensuring optimized binding interactions.
View Article and Find Full Text PDFMultifunctional Scaffold Biosensor and Drug Delivery System for Bacterial Infection Prevention During Skin Wound Healing.
Macromol Biosci
September 2025
IMEM-BRT Group, Departament d'Enginyeria Química, EEBE, Universitat Politècnica de Catalunya, Barcelona, Spain.
This study investigates a multifunctional hydrogel system integrating carboxymethyl cellulose (CMC) in a 3D-printed limonene (LIM) scaffold coated with poly(3,4-ethylenedioxythiophene): polystyrene sulfonate (PEDOT:PSS). The system allows to enhance wound healing, prevent infections, and monitor the healing progress. CMC is crosslinked with citric acid (CA) to form the hydrogel matrix (CMC-CA), while the 3D-printed limonene (LIM) scaffold is embedded within the hydrogel to provide mechanical support.
View Article and Find Full Text PDFZirconium ferrite nanoparticles as smart materials for energy and environmental applications: fractional-order supercapacitors, reservoirs of F ions, and efficient electrocatalysts for water splitting.
Nanoscale Adv
August 2025
School of Electronic Science, Odisha University of Technology and Research Bhubaneswar India.
A novel electrocatalyst, zirconium ferrite nanoparticles (NPs) (ZrFeO NPs), was synthesized through coprecipitation and calcination processes at 300 °C and 500 °C using iron rust. The ZrFeO NPs were used as catalysts for the hydrogen evolution reaction. Furthermore, these NPs in an alkaline medium exhibited superior properties of a fractional order supercapacitor, based on which a prototype device was fabricated to demonstrate its energy storage applications.
View Article and Find Full Text PDF