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Efficient information processing in the human brain is achieved by dynamics of neurons and synapses, motivating effective implementation of artificial spiking neural networks. Here, the dynamics of spin-orbit torque switching in antiferromagnet/ferromagnet heterostructures is studied to show the capability of the material system to form artificial neurons and synapses for asynchronous spiking neural networks. The magnetization switching, driven by a single current pulse or trains of pulses, is examined as a function of the pulse width (1 s to 1 ns), amplitude, number, and pulse-to-pulse interval. Based on this dynamics and the unique ability of the system to exhibit binary or analog behavior depending on the device size, key functionalities of a synapse (spike-timing-dependent plasticity) and a neuron (leaky integrate-and-fire) are reproduced in the same material and on the basis of the same working principle. These results open a way toward spintronics-based neuromorphic hardware that executes cognitive tasks with the efficiency of the human brain.
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http://dx.doi.org/10.1002/adma.201900636 | DOI Listing |
Phys Rev Lett
August 2025
University of Delaware, Department of Physics and Astronomy, Newark, Delaware 19716, USA.
Ultrafast light-driven strongly correlated antiferromagnetic insulators, such as prototypical NiO with a large Mott energy gap ≃4 eV, have recently attracted experimental attention using photons of both subgap [H. Qiu et al., Nat.
View Article and Find Full Text PDFJ Chem Theory Comput
September 2025
Institute of Theoretical Chemistry, Faculty of Chemistry, University of Vienna, Währinger Straße 17, 1090 Vienna, Austria.
We present a novel, flexible framework for electronic structure interfaces designed for nonadiabatic dynamics simulations, implemented in Python 3 using concepts of object-oriented programming. This framework streamlines the development of new interfaces by providing a reusable and extendable code base. It supports the computation of energies, gradients, various couplings─like spin-orbit couplings, nonadiabatic couplings, and transition dipole moments─and other properties for an arbitrary number of states with any multiplicities and charges.
View Article and Find Full Text PDFPhys Chem Chem Phys
September 2025
Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province, Shantou University, Shantou 515063, P. R. China.
The photophysical properties of two new Bodipy dimers are investigated using a variety of techniques, including steady-state UV-vis absorption and fluorescence spectroscopy, femtosecond and nanosecond transient absorption spectroscopy, and pulse laser-excited time-resolved electron paramagnetic resonance (TREPR) spectroscopic methods. The dimers are formed by the Bodipy units rigidly linked by the orthogonal phenylene bridge. One of the dimers is composed of iodinated units, and the other is not.
View Article and Find Full Text PDFSmall
September 2025
Department of Applied Biology and Chemical Technology and Research Institute for Smart Energy, The Hong Kong Polytechnic University, Hong Kong, 999077, P. R. China.
The precise modulation of the lifetime and the responsive properties of room-temperature phosphorescence (RTP) is essential for realizing its multifunctional applications. Herein, a facile strategy is presented to achieve a series of cellulose benzoate esters (CBE-X, X = H/CH/OH/NH) with lifetime-tunable RTP through substituent engineering. Enhancing the electron-donating ability of CBE-X effectively modulates the HOMO-LUMO gap, exciton energy, spin-orbit coupling, and interaction between cellulose chains, thereby enabling control over the RTP lifetime.
View Article and Find Full Text PDFJ Phys Chem Lett
September 2025
Department of Chemistry and Biochemistry, University of California, Los Angeles, California 90095, United States.
Biomolecules that constitute life on Earth are chiral, but the precise mechanism by which homochirality emerged remains a mystery. In this work, it is demonstrated that reactions of radical pairs, where one of the radical electron spins is polarized, can be enantioselective. This phenomenon arises from transient coherent quantum dynamics of the radical pair electron spins, which is known to occur even in warm and noisy condensed phase environments, where energetic perturbations much smaller than thermal energy can have strong effects on reactivity.
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