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Twisted light carrying orbital angular momentum (OAM) provides an additional degree of freedom for modern optics and an emerging resource for both classical and quantum information technologies. Its inherently infinite dimensions can potentially be exploited by using mode multiplexing to enhance data capacity for sustaining the unprecedented growth in big data and internet traffic and can be encoded to build large-scale quantum computing machines in high-dimensional Hilbert space. While the emission of twisted light from the surface of integrated devices to free space has been widely investigated, the transmission and processing inside a photonic chip remain to be addressed. Here, we present the first laser-direct-written waveguide being capable of supporting OAM modes and experimentally demonstrate a faithful mapping of twisted light into and out of a photonic chip. The states OAM_{0}, OAM_{-1}, OAM_{+1}, and their superpositions can transmit through the photonic chip with a total efficiency up to 60% with minimal crosstalk. In addition, we present the transmission of quantum twisted light states of single photons and measure the output states with single-photon imaging. Our results may add OAM as a new degree of freedom to be transmitted and manipulated in a photonic chip for high-capacity communication and high-dimensional quantum information processing.
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http://dx.doi.org/10.1103/PhysRevLett.121.233602 | DOI Listing |
Langmuir
September 2025
Biophysical Chemistry Laboratory, Physical Chemistry Section, Department of Chemistry, Jadavpur University, Raja S. C. Mullick Road, Jadavpur, Kolkata 700032, India.
Photophysical studies on the interaction of small molecules with various forms of nucleic acids are attracting attention nowadays in order to delineate the molecular level mechanism of various biological processes occurring in vivo. Herein, we employed vivid steady-state and time-resolved spectroscopic techniques to elucidate the detailed characterization of the binding interaction of a biologically active cationic dye thioflavin T (ThT) with double and triple helical forms of RNA - A.U duplex and U.
View Article and Find Full Text PDFNat Mater
September 2025
Department of Physics, University of Colorado, Boulder, CO, USA.
Time crystals are unexpected states of matter that spontaneously break time-translation symmetry either in a discrete or continuous manner. However, spatially mesoscale space-time crystals that break both space and time symmetries have not been reported. Here we report a continuous space-time crystal in a nematic liquid crystal driven by ambient-power, constant-intensity unstructured light.
View Article and Find Full Text PDFAdv Mater
September 2025
Department of Chemical Engineering, University of Michigan, Ann Arbor, MI, 48109, USA.
Metal-halide perovskites are known for their strong and tunable luminescence. However, the synthesis of perovskite-based particles with circularly polarized light emission (CPLE) remains challenging due to the complex interplay of metal-ligand chemistries, crystallization patterns, and chirality transfer mechanisms. Achiral perovskites can be deposited on chiral "hedgehog" particles (CHIPs) with twisted spikes, producing chiroptically active materials with spectroscopic bands specific to the perovskite and chirality specific to the template CHIPs.
View Article and Find Full Text PDFNanophotonics
August 2025
Departament de Física de la Matèria Condensada, Universitat de Barcelona, 08028 Barcelona, Spain.
We present a systematic investigation of the optical response to circularly polarized illumination in twisted stacked plasmonic nanostructures. The system consists in two identical, parallel gold triskelia, centrally aligned and rotated at a certain angle relative to each other. Sample fabrication was accomplished through a novel multilevel high-resolution electron beam lithography.
View Article and Find Full Text PDFChemPhotoChem
March 2025
Max Planck Research Group, Faculty of Chemistry and Pharmacy, Universidad del Atlántico, Barranquilla, 081007, Colombia.
Azocompounds are among the most important group of molecular photoswitches due to their multiple applications in various scientific areas. We studied the thermal and photochemical reactions of an azocompound with photo-induced antibiotic properties using calculations based on Kohn-Shan, Spin-Flip and time-dependent Density Functional Theory. Our primary goal is to understand the absorption spectra and isomerization pathways governing the molecule's light-controlled antibiotic activity.
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