Atmospheric biogenic volatile organic compounds in the Alaskan Arctic tundra: constraints from measurements at Toolik Field Station.

The Arctic is a climatically sensitive region that has experienced warming at almost 3 times the global average rate in recent decades, leading to an increase in Arctic greenness and a greater abundance of plants that emit biogenic volatile organic compounds (BVOCs). These changes in atmospheric emissions are expected to significantly modify the overall oxidative chemistry of the region and lead to changes in VOC composition and abundance, with implications for atmospheric processes. Nonetheless, observations needed to constrain our current understanding of these issues in this critical environment are sparse.

Constraining Emissions of Volatile Organic Compounds Over the Indian Subcontinent Using Space-Based Formaldehyde Measurements.

India is an air pollution mortality hot spot, but regional emissions are poorly understood. We present a high-resolution nested chemical transport model (GEOS-Chem) simulation for the Indian subcontinent and use it to interpret formaldehyde (HCHO) observations from two satellite sensors (OMI and GOME-2A) in terms of constraints on regional volatile organic compound (VOC) emissions. We find modeled biogenic VOC emissions to be overestimated by ~30-60% for most locations and seasons, and derive a best estimate biogenic flux of 16 Tg C/year subcontinent-wide for year 2009.

Source influence on emission pathways and ambient PM pollution over India (2015-2050).

India is currently experiencing degraded air quality, and future economic development will lead to challenges for air quality management. Scenarios of sectoral emissions of fine particulate matter and its precursors were developed and evaluated for 2015-2050, under specific pathways of diffusion of cleaner and more energy-efficient technologies. The impacts of individual source sectors on PM concentrations were assessed through systematic simulations of spatially and temporally resolved particulate matter concentrations, using the GEOS-Chem model, followed by population-weighted aggregation to national and state levels.

Aerosol Optical Depth Over India.

Tropospheric aerosol optical depth (AOD) over India was simulated by Goddard Earth Observing System (GEOS)-Chem, a global 3-D chemical-transport model, using SMOG (Speciated Multi-pOllutant Generator from Indian Institute of Technology Bombay) and GEOS-Chem (GC) (current inventories used in the GEOS-Chem model) inventories for 2012. The simulated AODs were ~80% (SMOG) and 60% (GC) of those measured by the satellites (Moderate Resolution Imaging Spectroradiometer and Multi-angle Imaging SpectroRadiometer). There is no strong seasonal variation in AOD over India.