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Physics-driven acoustic metamaterials offer unprecedented capabilities in manipulating sound wave propagation. Among these, sound-absorbing metamaterials emerge as powerful tools for achieving subwavelength control and high-efficiency absorption. However, most existing designs are typically constrained to unidirectional absorption, limiting their applicability in noise-sensitive scenarios requiring bidirectional control. Here, a switchable bidirectional acoustic metastructure is presented, integrating interleaved resonator coupling with exceptional point (EP) modulation. By coordinating vertical and horizontal resonant interactions through tailored impedance matching and controlled energy dissipation, the system achieves broadband and frequency-selective absorption in both directions-validated through theoretical, numerical, and experimental analyses. Specifically, broadband absorption from 478 to 670 Hz and discrete peaks at 260 and 542 Hz under opposite incidences are observed within the deep-subwavelength scale. Compared to state-of-the-art unidirectional absorbers, the proposed structure maintains geometric compactness while delivering robust bidirectional performance. Beyond device-level innovation, a generalized theoretical framework is developed to translate the effective acoustic parameters of resonance-based metastructures into specific impedance forms, enabling integration into EP-based switching strategies. This enables the functional extension from unidirectional to bidirectional absorption across a wide range of metastructures. Overall, this work offers a novel physics-driven pathway toward practical, high-performance, and bidirectional acoustic wave control.
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http://dx.doi.org/10.1002/advs.202508951 | DOI Listing |
Anal Methods
September 2025
Shenzhen Key Laboratory for Nano-Biosensing Technology, School of Biomedical Engineering, Shenzhen University Medical School, Shenzhen University, Shenzhen 518060, China.
Self-assembly is regarded as a facile method to fabricate luminescent nanomaterials with aggregation induced emission (AIE) properties for optical sensor design. In this work, a pH-controlled self-ratiometric sensing platform utilizing aggregation-induced emission (AIE)-active Au(I)-TCEP-Cd(II) nanoaggregates was developed for highly reliable D-penicillamine (DPA) detection. Through stoichiometric coordination with Cd, oligomeric Au(I)-tris(2-carboxyethyl)phosphine (TCEP) complexes could self-assemble into snowflake-like nanoaggregates (∼100 nm) with strong yellow emission (540 nm) and excellent aqueous stability.
View Article and Find Full Text PDFJ Am Chem Soc
August 2025
Research Institute for Electronic Science, Hokkaido University, Sapporo 001-0020, Japan.
Among various azoheteroarenes, thiazolylazo derivatives have recently emerged as bidirectional visible-light switches. However, their widespread application as molecular photoswitches remains limited due to synthetic challenges like robust reaction conditions, lack of commercial availability of starting material, and low reaction yield. This work presents a straightforward one-pot methodology for synthesizing thiazolylazo derivatives by reacting 2-trimethylsilylthiazole with various diazonium salts.
View Article and Find Full Text PDFAdv Sci (Weinh)
August 2025
School of Mechanical and Aerospace Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore, 639798, Singapore.
Physics-driven acoustic metamaterials offer unprecedented capabilities in manipulating sound wave propagation. Among these, sound-absorbing metamaterials emerge as powerful tools for achieving subwavelength control and high-efficiency absorption. However, most existing designs are typically constrained to unidirectional absorption, limiting their applicability in noise-sensitive scenarios requiring bidirectional control.
View Article and Find Full Text PDFACS Appl Mater Interfaces
June 2025
School of Physical Science and Technology, ShanghaiTech University, 393 Huaxia Middle Road, Pudong, Shanghai 201210, China.
Polymer-based soft actuators capable of responsive shape morphing hold great potential for developing untethered soft robotics with dexterous motion under complex surroundings. To realize this potential, achieving fast, dynamically tunable shape morphing that can generate sufficient mechanical force is essential. Here, soft actuators composed of liquid crystal elastomer (LCE) bilayer film are constructed via direct ink writing (DIW), which exhibit rapid and sequential 3D-to-3D́ morphological reconfiguration within seconds under temperature stimulus.
View Article and Find Full Text PDFNat Commun
May 2025
Terahertz Technology Innovation Research Institute, University of Shanghai for Science and Technology, Shanghai, China.
Information security aims to protect confidentiality and prevent information leakage, which inherently conflicts with the goal of information sharing. Balancing these competing requirements is especially challenging in all-optical systems, where efficient data transmission and rigorous security are essential. Here we propose and experimentally demonstrate a metasurface-based approach that integrates phase manipulation, polarization conversion, as well as direction- and polarization-selective functionalities into all-optical diffractive neural networks (DNNs).
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